Citation: QUAN Quan, XIE Shun-Ji, WANG Ye, XU Yi-Jun. Photoelectrochemical Reduction of CO₂ Over Graphene-Based Composites:Basic Principle,Recent Progress,and Future Perspective[J]. Acta Physico-Chimica Sinica, ;2017, 33(12): 2404-2423. doi: 10.3866/PKU.WHXB201706263 shu

Photoelectrochemical Reduction of CO₂ Over Graphene-Based Composites:Basic Principle,Recent Progress,and Future Perspective

QUAN Quan ^1, ,
XIE Shun-Ji ² ,
WANG Ye ² ,
XU Yi-Jun ¹

1.
State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou 350116, P. R. China;
2.
State Key Laboratory of Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, Fujian Province, P. R. China

Received Date: 5 June 2017
Revised Date: 19 June 2017

Fund Project: The project was supported by the National Natural Science Foundation of China (U1463204, 20903023 and 21173045), the Award Program for Minjiang Scholar Professorship, the Natural Science Foundation of Fujian Province for Distinguished Young Investigator Grant (2012J06003), the Independent Research Project of State Key Laboratory of Photocatalysis on Energy and Environment (2014A05), the first Program of Fujian Province for Top Creative Young Talents, the Open Research Project of State Key Laboratory of Physical Chemistry of Solid Surfaces of Xiamen University (201519), the Program for Returned High-Level Overseas Chinese Scholars of Fujian province, and the Natural Science Foundation of Fujian Province for Distinguished Young Investigator Rolling Grant (2017J07002).

In response to aggravated fossil resources consuming and greenhouse effect, CO₂ reduction has become a globally important scientific issue because this method can be used to produce value-added feedstock for application in alternative energy supply. Photoelectrocatalysis, achieved by combining optical energy and external electrical bias, is a feasible and promising system for CO₂ reduction. In particular, applying graphene in tuning photoelectrochemical CO₂ reduction has aroused considerable attention because graphene is advantageous for enhancing CO₂ adsorption, facilitating electrons transfer, and thus optimizing the performance of graphene-based composite electrodes. In this review, we elaborate the fundamental principle, basic preparation methods, and recent progress in developing a variety of graphene-based composite electrodes for photoelectrochemical reduction of CO₂ into solar fuels and chemicals. We also present a perspective on the opportunities and challenges for future research in this booming area and highlight the potential evolution strategies for advancing the research on photoelectrochemical CO₂ reduction.
- Photoelectrochemical,
- CO₂ reduction,
- Graphene-based composite
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

Photoelectrochemical Reduction of CO2 Over Graphene-Based Composites:Basic Principle,Recent Progress,and Future Perspective

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通讯作者: 陈斌, bchen63@163.com

Photoelectrochemical Reduction of CO₂ Over Graphene-Based Composites:Basic Principle,Recent Progress,and Future Perspective