Citation: ZHUANG Jian-Dong, TIAN Qin-Fen, LIU Ping. Bi₂Sn₂O₇ Visible-Light Photocatalysts: Different Hydrothermal Preparation Methods and Their Photocatalytic Performance for As(Ⅲ) Removal[J]. Acta Physico-Chimica Sinica, ;2016, 32(2): 551-557. doi: 10.3866/PKU.WHXB201511304 shu

Bi₂Sn₂O₇ Visible-Light Photocatalysts: Different Hydrothermal Preparation Methods and Their Photocatalytic Performance for As(Ⅲ) Removal

1.
1 College of Materials Engineering, Fujian Agriculture and Forestry University, Fuzhou 350002, P. R. China;
2.
2 State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou 350002, P. R. China

Corresponding author: ZHUANG Jian-Dong,
Received Date: 6 October 2015
Available Online: 26 November 2015
Fund Project: 国家自然科学基金(21303244) (21303244)福建农林大学杰出青年基金(XJQ201419)资助项目 (XJQ201419)

Bi₂Sn₂O₇, synthesized through different hydrothermal routes (the microwave hydrothermal method (MH-BSO) and the traditional hydrothermal method (TH-BSO)), was used for photocatalytic removal of arsenic from aqueous solution. The as-synthesized Bi₂Sn₂O₇ products were characterized by X-ray diffraction (XRD), N2 sorption-desorption, UV-Vis diffuse reflectance spectroscopy (UV-Vis DRS), transmission electron microscopy (TEM), electron spin resonance (ESR), X-ray photoelectron spectra (XPS), and electrochemistry technology. Under visible light irradiation, the MH-BSO sample exhibited a higher photocatalytic activity (up to 98.7%) than that of the TH-BSO sample during the oxidization of arsenite (AsO₃)^3-. The active species, O₂^-· and h_VB⁺, were identified as the primary active species responsible for As(Ⅲ) oxidation. In addition, a possible mechanism for the photo-oxidation of As(Ⅲ) over Bi₂Sn₂O₇ is proposed.
- Bi₂Sn₂O₇,
- Microwave hydrothermal method,
- Traditional hydrothermal method,
- Visible-light photocatalysis,
- As(Ⅲ) oxidation
1. [1]
  (1) Amini, M.; Mueller, K.; Abbaspour, K. C.; Rosenberg, T.; Afyuni, M.; Mø ller, K. N.; Sarr, M.; Johnson, C. A.Environmental Science & Technology 2008, 42, 3662. doi: 10.1021/es071958y
2. [2]
  (2) Welch, A. H.; Westjohn, D.; Helsel, D. R.; Wanty, R. B. Ground Water 2000, 38, 589. doi: 10.1111/gwat.2000.38.issue-4
3. [3]
  (3) Kumar Maji, S.; Pal, A. Recent Patents on Engineering 2010, 4, 92. doi: 10.2174/187221210791233461
4. [4]
  (4) Lee, H.; Choi, W. Environmental Science & Technology 2002, 36, 3872. doi: 10.1021/es0158197
5. [5]
  (5) Kim, Y.; Kim, C.; Choi, I.; Rengaraj, S.; Yi, J. Environmental Science & Technology 2004, 38, 924. doi: 10.1021/es0346431
6. [6]
  (6) Bissen, M.; Frimmel, F. H. Acta Hydrochimica et Hydrobiologica 2003, 31, 9. doi: 10.1002/aheh.200390025
7. [7]
  (7) Bissen, M.; Frimmel, F. H. Acta Hydrochimica et Hydrobiologica 2003, 31, 97.
8. [8]
  (8) Driehaus, W.; Seith, R.; Jekel, M. Water Research 1995, 29, 297. doi: 10.1016/0043-1354(94)E0089-O
9. [9]
  (9) Emett, M. T.; Khoe, G. H. Water Research 2001, 35, 649. doi: 10.1016/S0043-1354(00)00294-3
10. [10]
  (10) Pettine, M.; Campanella, L.; Millero, F. J. Geochimica et Cosmochimica Acta 1999, 63, 2727. doi: 10.1016/S0016-7037(99)00212-4
11. [11]
  (11) Kim, M. J.; Nriagu, J. Science of the Total Environment 2000, 247, 71. doi: 10.1016/S0048-9697(99)00470-2
12. [12]
  (12) Bissen, M.; Vieillard-Baron, M. M.; Schindelin, A. J.; Frimmel, F. H. Chemosphere 2001, 44, 751. doi: 10.1016/S0045-6535(00)00489-6
13. [13]
  (13) Dutta, P. K.; Pehkonen, S.; Sharma, V. K.; Ray, A. K.Environmental Science & Technology 2005, 39, 1827. doi: 10.1021/es0489238
14. [14]
  (14) Fostier, A. H.; Pereira, M. D. S. S.; Rath, S.; Guimarã es, J. R.Chemosphere 2008, 72, 319. doi: 10.1016/j.chemosphere.2008.01.067
15. [15]
  (15) Xu, T.; Cai, Y.; O'Shea, K. E. Environmental Science & Technology 2007, 41, 5471. doi: 10.1021/es0628349
16. [16]
  (16) Ló pez-Muñ oz, M.; Revilla, A.; Alcalde, G. Catalysis Today 2015, 240, 138. doi: 10.1016/j.cattod.2014.05.008
17. [17]
  (17) Yang, H.; Lin, W. Y.; Rajeshwar, K. Journal of Photochemistry and Photobiology A: Chemistry 1999, 123, 137. doi: 10.1016/S1010-6030(99)00052-0
18. [18]
  (18) Ryu, J.; Choi, W. Environmental Science & Technology 2004, 38, 2928. doi: 10.1021/es034725p
19. [19]
  (19) Devi, G. S.; Manorama, S.; Rao, V. Journal of the Electrochemical Society 1998, 145, 1039. doi: 10.1149/1.1838385
20. [20]
  (20) Udod, L.; Aplesnin, S.; Sitnikov, M.; Molokeev, M. Physics of the Solid State 2014, 56, 1315. doi: 10.1134/S1063783414070336
21. [21]
  (21) Andrews, P. C.; Junk, P. C.; Nuzhnaya, I.; Thielemann, D. T.Inorganic Chemistry 2012, 51, 751. doi: 10.1021/ic202707p
22. [22]
  (22) Du, S. Q.; Yuan, Y. F.; Tu, W. X. Acta Phys. -Chim. Sin. 2013, 29 (9), 2062. [杜书青, 袁宇峰, 涂伟霞. 物理化学学报, 2013, 29(9), 2062.] doi: 10.3866/PKU.WHXB201306213
23. [23]
  (23) Tian, Q.; Zhuang, J.; Wang, J.; Liu, P. Applied Catalysis A: General 2012, 425, 74.
24. [24]
  (24) Nesbitt, H.; Canning, G.; Bancroft, G. Geochimica et Cosmochimica Acta 1998, 62, 2097. doi: 10.1016/S0016-7037(98)00146-X
25. [25]
  (25) Liu, G.; Zhao, J.; Hidaka, H. Journal of Photochemistry and Photobiology A: Chemistry 2000, 133, 83. doi: 10.1016/S1010-6030(00)00227-6
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Bi₂Sn₂O₇ Visible-Light Photocatalysts: Different Hydrothermal Preparation Methods and Their Photocatalytic Performance for As(Ⅲ) Removal