Citation: CHEN Feng-Ying, XIAO Li, YANG Cui-Xia, ZHUANG Lin. Preparation and Electrocatalytic Properties of Perovskite Type Oxides CaVO₃ for Oxygen Reduction Reaction[J]. Acta Physico-Chimica Sinica, ;2015, 31(12): 2310-2315. doi: 10.3866/PKU.WHXB201510162 shu

Preparation and Electrocatalytic Properties of Perovskite Type Oxides CaVO₃ for Oxygen Reduction Reaction

CHEN Feng-Ying ^1,2 ,
XIAO Li ^1,, ,
YANG Cui-Xia ¹ ,
ZHUANG Lin ^1,,

1.
1 College of Chemistry and Molecular Sciences, Wuhan University, Wuhan 430072, P. R. China;
2.
2 College of Chemical Engineering and Modern Materials/Shaanxi Key Laboratory of Comprehensive Utilization of Tailings Resources, Shangluo University, Shangluo 726000, Shaanxi Province, P. R. China

Corresponding author: XIAO Li, ZHUANG Lin,
Received Date: 13 July 2015
Available Online: 15 October 2015
Fund Project: 国家自然科学基金(21273171) (21273171)商洛市科技计划基金(SK2014-01-09)资助项目 (SK2014-01-09)

The precursor powder of CaVO₃ was prepared by sol-gel method using vanadium pentoxide, calcium nitrate, citric acid, and oxalic acid as raw materials. The target product CaVO₃ was obtained by calcining the precursor powder in argon atmosphere at 1000 ℃. In order to determine the appropriate calcination temperature, thermal stability of the precursor powder was tested. The target product CaVO₃ was characterized by Fourier transform infrared (FTIR) spectrometry, thermogravimetry (TG), X-ray diffraction (XRD), and conductivity. In addition, the properties for oxygen reduction reaction (ORR) were also investigated, and the results showed that the electron transfer number of ORR on the modified electrode was 1.5-1.7, which indicating that ORR was a two-electron process.
- Perovskite,
- Sol-gel method,
- Oxygen reduction reaction
1. [1]
  (1) Gallego, G. S.; Mondracn, F.; Barrault, J.; Tatibouet, J. M.; Batiot-Dupeyrat, C. Appl. Catal. A 2006, 311, 164. doi: 10.1016/j.apcata.2006.06.024
2. [2]
  (2) Derrama, G.; Kiennemann, A.; Gold, A. R. J. Power Sources 2010, 195 (7), 1765. doi: 10.1016/j.jpowsour.2009.10.004
3. [3]
  (3) Choi, S. O.; Moon, S. H. Catal. Today 2009, 146 (1-2), 148. doi: 10.1016/j.cattod.2009.02.023
4. [4]
  (4) Petrovica, S.; Rarae, V.; Jovanowd, D. M.; Barieevie, A. T. Appl. Catal. 2006, 66 (3-4), 249. doi: 10.1016/j.apcatb.2006.04.003
5. [5]
  (5) Bulgan, G.; Teng, F.; Liang, S. H.; Yao, W. Q.; Zhu, Y. Ｆ. Acta Phys. -Chim. Sin. 2007, 23 (9), 1387. [Bulgan G, 滕飞, 梁淑惠, 姚文清, 朱永法. 物理化学学报, 2007, 23 (9), 1387.] doi: 10.3866/PKU.WHXB20070915
6. [6]
  (6) Rida, K.; Benabbas, A.; Bouremmad, F.; Pena, M. A.; Sastre, E.; Martinez, A. A. Appl. Catal. A 2007, 327 (2), 173. doi: 10.1016/j.apcata.2007.05.015
7. [7]
  (7) Iojoiu, E. E.; Bassou, B.; Guilhaume, N.; Farrusseng, D.; Desmailtin, C. A.; Lombaert, K.; Bianchi, D.; Mirodatos, C. Catal. Today 2008, 137 (1), 103. doi: 10.1016/j.cattod.2008.02.016
8. [8]
  (8) Wang, Y. Q.; Hu, R. S.; Wu, P.; Su, H. Q. Ind. Catal. 2006, 14 (3), 56. [王宴秋, 胡瑞生, 武鹏, 苏海全. 工业催化, 2006, 14 (3), 56.]
9. [9]
  (9) Stathopoulos, V. N.; Belessi, V. C.; Bakas, T. V.; Neophytides, S. G.; Costa, C. N.; Pomonis, P. J.; Efstathiou, A. M. Appl. Catal. B 2009, 93 (1-2), 1. doi: 10.1016/j.apcatb.2009.09.003
10. [10]
  (10) Zhu, Y. J.; Wang, D.; Yuan, F. L.; Zhang, G.; Fu, H. G. Appl. Catal. 2008, 82 (3-4), 255. doi: 10.1016/j.apcatb.2008.01.025
11. [11]
  (11) Zhu, J. J.; Thomas, A. Appl. Catal. B 2009, 92 (3-4), 225. doi: 10.1016/j.apcatb.2009.08.008
12. [12]
  (12) Barbero, B. P.; Gamboa, J A.; Cados, L. E. Appl. Catal. B 2006, 65 (1-2), 21. doi: 10.1016/j.apcatb.2005.11.018
13. [13]
  (13) Li, W. B.; Wang, J. X.; Gong, H. Catal. Today 2009, 148 (1-2), 81. doi: 10.1016/j.cattod.2009.03.007
14. [14]
  (14) Balasubramanian, A.; Karthikeyan, N.; Giridhar, V. V. J. Power Sources 2008, 185 (2), 670. doi: 10.1016/j.jpowsour.2008.08.096
15. [15]
  (15) Kishori, D.; Alexander, M.; Arvind, V. J. Power Sources 2006, 158 (1), 60. doi: 10.1016/j.jpowsour.2005.09.025
16. [16]
  (16) Hammouche, A.; Kahoul, A.; Sauer, D. U.; De Doncker, R. W. J. Power Sources 2006, 153 (2), 239. doi: 10.1016/j.jpowsour.2005.05.028
17. [17]
  (17) Singh, R. N.; Aninditam, M.; Sinha, A. S. K.; Chartier, P. Electrochimi. Acta 2007, 52 (12), 4264. doi: 10.1016/j.electacta.2006.12.004
18. [18]
  (18) Chang, Y. M.; Wu, P. W.; Wu, C. Y.; Hsieh, Y. C. J. Power Sources 2009, 189 (2), 1003. doi: 10.1016/j.jpowsour.2008.12.101
19. [19]
  (19) Yasutake, T.; Hirofumi, K.; Isamu, M. Chem. Lett. 1991, 20 (4), 673.
20. [20]
  (20) Chamberland, B. L.; Danielson, P. S. J. Solid State Chem. 1971, 3 (2), 243. doi: 10.1016/0022-4596(71)90035-1
21. [21]
  (21) Falcó n, H.; Alonso, J. A.; Casais, M. T.; Martí nez-Lope, M. J.; Sá nchez-Bení tez, J. J. Solid State Chem. 2004, 177 (9), 3099. doi: 10.1016/j.jssc.2004.05.010
22. [22]
  (22) Yutaka, U. J. Solid State Chem. 1998, 135 (1), 36. doi: 10.1006/jssc.1997.7587
23. [23]
  (23) Jiang, R. Z.; Anson, F. C. J. Electroanal. Chem. 1991, 305 (1), 171.
24. [24]
  (24) Tammeveski, K.; Tenno, T.; Claret, J.; Ferrater, C. Electrochim. Acta 1997, 42 (5), 893. doi: 10.1016/S0013-4686(96)00325-8
1. [1]
  Lin Song , Dourong Wang , Biao Zhang . Innovative Experimental Design and Research on Preparing Flexible Perovskite Fluorescent Gels Using 3D Printing. University Chemistry, 2024, 39(7): 337-344. doi: 10.3866/PKU.DXHX202310107
2. [2]
  Yixuan Gao , Lingxing Zan , Wenlin Zhang , Qingbo Wei . Comprehensive Innovation Experiment: Preparation and Characterization of Carbon-based Perovskite Solar Cells. University Chemistry, 2024, 39(4): 178-183. doi: 10.3866/PKU.DXHX202311091
3. [3]
  Cheng PENG , Jianwei WEI , Yating CHEN , Nan HU , Hui ZENG . First principles investigation about interference effects of electronic and optical properties of inorganic and lead-free perovskite Cs₃Bi₂X₉ (X=Cl, Br, I). Chinese Journal of Inorganic Chemistry, 2024, 40(3): 555-560. doi: 10.11862/CJIC.20230282
4. [4]
  Rui Li , Huan Liu , Yinan Jiao , Shengjian Qin , Jie Meng , Jiayu Song , Rongrong Yan , Hang Su , Hengbin Chen , Zixuan Shang , Jinjin Zhao . 卤化物钙钛矿的单双向离子迁移. Acta Physico-Chimica Sinica, 2024, 40(11): 2311011-. doi: 10.3866/PKU.WHXB202311011
5. [5]
  Xinyuan Shi , Chenyangjiang , Changyu Zhai , Xuemei Lu , Jia Li , Zhu Mao . Preparation and Photoelectric Performance Characterization of Perovskite CsPbBr₃ Thin Films. University Chemistry, 2024, 39(6): 383-389. doi: 10.3866/PKU.DXHX202312019
6. [6]
  Fan JIA , Wenbao XU , Fangbin LIU , Haihua ZHANG , Hongbing FU . Synthesis and electroluminescence properties of Mn²⁺ doped quasi-two-dimensional perovskites (PEA)₂Pb_yMn_1-yBr₄. Chinese Journal of Inorganic Chemistry, 2024, 40(6): 1114-1122. doi: 10.11862/CJIC.20230473
7. [7]
  Zeyuan WANG , Songzhi ZHENG , Hao LI , Jingbo WENG , Wei WANG , Yang WANG , Weihai SUN . Effect of I₂ interface modification engineering on the performance of all-inorganic CsPbBr₃ perovskite solar cells. Chinese Journal of Inorganic Chemistry, 2024, 40(7): 1290-1300. doi: 10.11862/CJIC.20240021
8. [8]
  Jizhou Liu , Chenbin Ai , Chenrui Hu , Bei Cheng , Jianjun Zhang . 六氯锡酸铵促进钙钛矿太阳能电池界面电子转移及其飞秒瞬态吸收光谱研究. Acta Physico-Chimica Sinica, 2024, 40(11): 2402006-. doi: 10.3866/PKU.WHXB202402006
9. [9]
  Hailang JIA , Hongcheng LI , Pengcheng JI , Yang TENG , Mingyun GUAN . Preparation and performance of N-doped carbon nanotubes composite Co₃O₄ as oxygen reduction reaction electrocatalysts. Chinese Journal of Inorganic Chemistry, 2024, 40(4): 693-700. doi: 10.11862/CJIC.20230402
10. [10]
  Xiaofeng Zhu , Bingbing Xiao , Jiaxin Su , Shuai Wang , Qingran Zhang , Jun Wang . Transition Metal Oxides/Chalcogenides for Electrochemical Oxygen Reduction into Hydrogen Peroxides. Acta Physico-Chimica Sinica, 2024, 40(12): 2407005-. doi: 10.3866/PKU.WHXB202407005
11. [11]
  Hui Shi , Shuangyan Huan , Yuzhi Wang . Ideological and Political Design of Potassium Permanganate Oxidation-Reduction Titration Experiment. University Chemistry, 2024, 39(2): 175-180. doi: 10.3866/PKU.DXHX202308042
12. [12]
  Zongfei YANG , Xiaosen ZHAO , Jing LI , Wenchang ZHUANG . Research advances in heteropolyoxoniobates. Chinese Journal of Inorganic Chemistry, 2024, 40(3): 465-480. doi: 10.11862/CJIC.20230306
13. [13]
  Yuena Yang , Xufang Hu , Yushan Liu , Yaya Kuang , Jian Ling , Qiue Cao , Chuanhua Zhou . The Realm of Smart Hydrogels. University Chemistry, 2024, 39(5): 172-183. doi: 10.3866/PKU.DXHX202310125
14. [14]
  Jinfeng Chu , Yicheng Wang , Ji Qi , Yulin Liu , Yan Li , Lan Jin , Lei He , Yufei Song . Comprehensive Chemical Experiment Design: Convenient Preparation and Characterization of an Oxygen-Bridged Trinuclear Iron(III) Complex. University Chemistry, 2024, 39(7): 299-306. doi: 10.3866/PKU.DXHX202310105
15. [15]
  Yunting Shang , Yue Dai , Jianxin Zhang , Nan Zhu , Yan Su . Something about RGO (Reduced Graphene Oxide). University Chemistry, 2024, 39(9): 273-278. doi: 10.3866/PKU.DXHX202306050
16. [16]
  Shengjuan Huo , Xiaoyan Zhang , Xiangheng Li , Xiangning Li , Tianfang Chen , Yuting Shen . Unveiling the Marvels of Titanium: Popularizing Multifunctional Colored Titanium Product Films. University Chemistry, 2024, 39(5): 184-192. doi: 10.3866/PKU.DXHX202310127
17. [17]
  Endong YANG , Haoze TIAN , Ke ZHANG , Yongbing LOU . Efficient oxygen evolution reaction of CuCo₂O₄/NiFe-layered bimetallic hydroxide core-shell nanoflower sphere arrays. Chinese Journal of Inorganic Chemistry, 2024, 40(5): 930-940. doi: 10.11862/CJIC.20230369
18. [18]
  Lu XU , Chengyu ZHANG , Wenjuan JI , Haiying YANG , Yunlong FU . Zinc metal-organic framework with high-density free carboxyl oxygen functionalized pore walls for targeted electrochemical sensing of paracetamol. Chinese Journal of Inorganic Chemistry, 2024, 40(5): 907-918. doi: 10.11862/CJIC.20230431
19. [19]
  Kun WANG , Wenrui LIU , Peng JIANG , Yuhang SONG , Lihua CHEN , Zhao DENG . Hierarchical hollow structured BiOBr-Pt catalysts for photocatalytic CO₂ reduction. Chinese Journal of Inorganic Chemistry, 2024, 40(7): 1270-1278. doi: 10.11862/CJIC.20240037
20. [20]
  Zhuo WANG , Junshan ZHANG , Shaoyan YANG , Lingyan ZHOU , Yedi LI , Yuanpei LAN . Preparation and photocatalytic performance of CeO₂-reduced graphene oxide by thermal decomposition. Chinese Journal of Inorganic Chemistry, 2024, 40(9): 1708-1718. doi: 10.11862/CJIC.20240067

Get Citation

PDF

XML

Metrics

PDF Downloads(24)
Abstract views(276)
HTML views(18)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142

Preparation and Electrocatalytic Properties of Perovskite Type Oxides CaVO3 for Oxygen Reduction Reaction

Metrics

通讯作者: 陈斌, bchen63@163.com

Preparation and Electrocatalytic Properties of Perovskite Type Oxides CaVO₃ for Oxygen Reduction Reaction