Citation: SUN Zhi-Guo, GAO Xiong-Hou, MA Jian-Tai, ZHANG Li, LIU Hong-Hai, WANG Bao-Jie. Effect of Lauryl Sodium Sulfate on the In situ Crystallization of Small-Grain NaY[J]. Acta Physico-Chimica Sinica, ;2015, 31(10): 2011-2015. doi: 10.3866/PKU.WHXB201508211 shu

Effect of Lauryl Sodium Sulfate on the In situ Crystallization of Small-Grain NaY

1.
1 Lanzhou Petrochemical Research Center, Petrochemical Research Institute, PetroChina, Lanzhou 730060, P. R. China;
2 College of Chemistry and Chemical Engineering, Lanzhou University, Lanzhou 730000, P. R. China

Received Date: 23 June 2015
Available Online: 21 August 2015
Fund Project: 中国石油天然气有限公司项目(2014A-2108)资助 (2014A-2108)

The in situ crystallization of small-grain NaY in the presence of lauryl sodium sulfate was investigated. The product containing small-grain NaY was used as a matrix to prepare REUSY catalyst via ammonium ion exchange and rare earth ion exchange. X-ray diffraction (XRD), scanning electron microscopy (SEM), X-ray fluorescence (XRF), and N₂ physical adsorption-desorption were used to characterize the samples, while the catalytic performance of prepared catalysts was evaluated by micro-activity evaluation device and advanced catalytic evaluation (ACE). It is indicated that the addition of lauryl sodium sulfate (5% of Kaolin microsphere mass) to in situ crystallization system can decrease the average grain size of the zeolite from 540 to 250 nm. Relative to the conventional in situ crystallization fluid catalytic cracking (FCC) catalysts, the catalyst prepared from in situ crystallization product containing small-grain NaY exhibits improved performance in the conversion rate of feedstock, the selectivity of the cracking product, and the resistance to carbon deposition.
- Small grain NaY,
- In situ crystallization,
- Lauryl sodium sulfate,
- Heavy oil,
- Fluid catalytic cracking
1. [1]
  
  (1) Sadeghbeigi, R. Fluid Catalytic Cracking Handbook: an Expert Guide to the Practical Operation, Design, and Optimization of FCC Units, 3rd ed.; Elsevier: Amsterdam, 2012; pp 1-42.
2. [2]
  (2) Chen, H. L.; Sheng, B. J.; Pan, H. F. Acta Phys. -Chim. Sin. 2004, 20 (8), 854. [陈洪林, 申宝剑, 潘惠芳. 物理化学学报, 2004, 20 (8), 854.] doi: 10.3866/PKU.WHXB20040814
3. [3]
  (3) García-Martínez, J.; Li, K.; Krishnaiah, G. Chem. Commun. 2012, 48 (97), 11841. doi: 10.1039/c2cc35659g
4. [4]
  (4) Cao, X. H. Pet. Process. Petroche. 2002, 33 (9), 1. [曹湘洪. 石油炼制与化工, 2002, 33, 1.]
5. [5]
  (5) Vuong, G. T.; Hoang, V. T.; Nguyen, D. T.; Do, T. O. Appl. Catal. A: Gen. 2010, 382 (2), 231. doi: 10.1016/j.apcata.2010.04.049
6. [6]
  (6) Mastropietro, T. F.; Drioli, E.; Poerio, T. RSC Adv. 2014, 4 (42), 21951. doi: 10.1039/c4ra03376k
7. [7]
  (7) Chaves, T. F.; Pastore, H. O.; Cardoso, D. Microporous Mesoporous Mat. 2012, 161, 67. doi: 10.1016/j.micromeso.2012.05.022
8. [8]
  (8) Larsen, S. C. J. Phys. Chem. C 2007, 111 (50), 18464. doi: 10.1021/jp074980m
9. [9]
  (9) Holmberg, B. A.; Wang, H.; Norbeck, J. M.; Yan, Y. S. Microporous Mesoporous Mat. 2003, 59 (1), 13. doi: 10.1016/S1387-1811(03)00271-3
10. [10]
  (10) Chao, Z. S.; Lin, H. Q.; Chen, G. Z.; Wu, T. H.; Wan, H. L.; Min, E. Z. Chem. J. Chin. Univ. 2000, 21 (9), 1353. [晁自胜, 林海强, 陈国周, 吴廷华, 万惠霖, 闵恩泽. 高等学校化学学报, 2000, 21 (9), 1353.]
11. [11]
  (11) Chao, Z. S.; Lin, H. Q.; Chen, G. Z.; Wu, T. H.; Wan, H. L.; Min, E. Z. Chem. J. Chin. Univ. 2001, 22 (1), 10. [晁自胜, 林海强, 陈国周, 吴廷华, 万惠霖, 闵恩泽. 高等学校化学学报, 2001, 22 (1), 10.]
12. [12]
  (12) Cheng, Z. L.; Chao, Z. S.; Wan, H. L. Acta Phys. -Chim. Sin. 2003, 19 (6), 487. [程志林, 晁自胜, 万惠霖. 物理化学学报, 2003, 19 (6), 487.] doi: 10.3866/PKU.WHXB20030602
13. [13]
  (13) Tang, K.; Wang, Y. G.; Song, L. J.; Duan, L. H.; Zhang, X. T.; Sun, Z. L. Mater. Lett. 2006, 60 (17), 2158.
14. [14]
  (14) Tan, J.; Chen, Y.; Liu, J.; Wang, Y. H. B. Chin. Ceram. Soc. 2011, 30 (1), 13. [谭涓, 陈颖, 刘靖, 王业红. 硅酸盐通报, 2011, 30 (1), 13.]
15. [15]
  (15) Tan, Q. F.; Bao, X. J.; Song, T. C.; Fan, Y.; Shi, G.; Shen, B. J.; Liu, C. H.; Gao, X. H. J. Catal. 2007, 251 (1), 69. doi: 10.1016/j.jcat.2007.07.014
16. [16]
  (16) Liu, H. H.; Zhao, H. J.; Gao, X. H.; Ma, J. T. Catal. Today 2007, 125 (3), 163.
17. [17]
  (17) Liu, H. H.; Ma, J. T.; Gao, X. H. Catal. Lett. 2006, 110 (3-4), 229. doi: 10.1007/s10562-006-0113-z
18. [18]
  (18) Khomane, R. B.; Kulkarni, B. D.; Ahedi, R. K. J. Colloid Interface Sci. 2001, 236, 208. doi: 10.1006/jcis.2000.7406
19. [19]
  (19) Iwakai, K.; Ta , T.; Konno, H.; Nakasaka, Y.; Masuda, T. Microporous Mesoporous Mat. 2011, 141, 167. doi: 10.1016/j.micromeso.2010.11.001
1. [1]
  Shiyan Cheng , Yonghong Ruan , Lei Gong , Yumei Lin . Research Advances in Friedel-Crafts Alkylation Reaction. University Chemistry, 2024, 39(10): 408-415. doi: 10.12461/PKU.DXHX202403024
2. [2]
  Wenyan Dan , Weijie Li , Xiaogang Wang . The Technical Analysis of Visual Software ShelXle for Refinement of Small Molecular Crystal Structure. University Chemistry, 2024, 39(3): 63-69. doi: 10.3866/PKU.DXHX202302060
3. [3]
  Zhifang SU , Zongjie GUAN , Yu FANG . Process of electrocatalytic synthesis of small molecule substances by porous framework materials. Chinese Journal of Inorganic Chemistry, 2024, 40(12): 2373-2395. doi: 10.11862/CJIC.20240290
4. [4]
  Yinyin Qian , Rui Xu . Utilizing VESTA Software in the Context of Material Chemistry: Analyzing Twin Crystal Nanostructures in Indium Antimonide. University Chemistry, 2024, 39(3): 103-107. doi: 10.3866/PKU.DXHX202307051
5. [5]
  Xin Han , Zhihao Cheng , Jinfeng Zhang , Jie Liu , Cheng Zhong , Wenbin Hu . Design of Amorphous High-Entropy FeCoCrMnBS (Oxy) Hydroxides for Boosting Oxygen Evolution Reaction. Acta Physico-Chimica Sinica, 2025, 41(4): 100033-. doi: 10.3866/PKU.WHXB202404023
6. [6]
  Wen YANG , Didi WANG , Ziyi HUANG , Yaping ZHOU , Yanyan FENG . La promoted hydrotalcite derived Ni-based catalysts: In situ preparation and CO₂ methanation performance. Chinese Journal of Inorganic Chemistry, 2024, 40(3): 561-570. doi: 10.11862/CJIC.20230276
7. [7]
  Jihua Deng , Xinshi Wu , Dichang Zhong . Exploration of Green Teaching and Ideological and Political Education in Chemical Experiment of “Preparation of Ammonium Ferrous Sulfate”. University Chemistry, 2024, 39(10): 325-329. doi: 10.12461/PKU.DXHX202405046
8. [8]
  Qin Li , Huihui Zhang , Huajun Gu , Yuanyuan Cui , Ruihua Gao , Wei-Lin Dai . In situ Growth of Cd_0.5Zn_0.5S Nanorods on Ti₃C₂ MXene Nanosheet for Efficient Visible-Light-Driven Photocatalytic Hydrogen Evolution. Acta Physico-Chimica Sinica, 2025, 41(4): 100031-. doi: 10.3866/PKU.WHXB202402016
9. [9]
  Guangming YIN , Huaiyao WANG , Jianhua ZHENG , Xinyue DONG , Jian LI , Yi'nan SUN , Yiming GAO , Bingbing WANG . Preparation and photocatalytic degradation performance of Ag/protonated g-C₃N₄ nanorod materials. Chinese Journal of Inorganic Chemistry, 2024, 40(8): 1491-1500. doi: 10.11862/CJIC.20240086
10. [10]
  Yufang GAO , Nan HOU , Yaning LIANG , Ning LI , Yanting ZHANG , Zelong LI , Xiaofeng LI . Nano-thin layer MCM-22 zeolite: Synthesis and catalytic properties of trimethylbenzene isomerization reaction. Chinese Journal of Inorganic Chemistry, 2024, 40(6): 1079-1087. doi: 10.11862/CJIC.20240036
11. [11]
  Lina Guo , Ruizhe Li , Chuang Sun , Xiaoli Luo , Yiqiu Shi , Hong Yuan , Shuxin Ouyang , Tierui Zhang . 层状双金属氢氧化物的层间阴离子对衍生的Ni-Al₂O₃催化剂光热催化CO₂甲烷化反应的影响. Acta Physico-Chimica Sinica, 2025, 41(1): 2309002-. doi: 10.3866/PKU.WHXB202309002
12. [12]
  Yifeng Xu , Jiquan Liu , Bin Cui , Yan Li , Gang Xie , Ying Yang . “Xiao Li’s School Adventures: The Working Principles and Safety Risks of Lithium-ion Batteries”. University Chemistry, 2024, 39(9): 259-265. doi: 10.12461/PKU.DXHX202404009
13. [13]
  Ziliang KANG , Jiamin ZHANG , Hong AN , Xiaohua LIU , Yang CHEN , Jinping LI , Libo LI . Preparation and water adsorption properties of CaCl₂@MOF-808 in-situ composite moulded particles. Chinese Journal of Inorganic Chemistry, 2024, 40(11): 2133-2140. doi: 10.11862/CJIC.20240282
14. [14]
  Zheqi Wang , Yawen Lin , Shunliu Deng , Huijun Zhang , Jinmei Zhou . Antiviral Strategies: A Brief Review of the Development History of Small Molecule Antiviral Drugs. University Chemistry, 2024, 39(9): 85-93. doi: 10.12461/PKU.DXHX202403108
15. [15]
  Hongsheng Tang , Yonghe Zhang , Dexiang Wang , Xiaohui Ning , Tianlong Zhang , Yan Li , Hua Li . A Wonderful Journey through the Kingdom of Hazardous Chemicals. University Chemistry, 2024, 39(9): 196-202. doi: 10.12461/PKU.DXHX202403098
16. [16]
  Qiuyang LUO , Xiaoning TANG , Shu XIA , Junnan LIU , Xingfu YANG , Jie LEI . Application of a densely hydrophobic copper metal layer in-situ prepared with organic solvents for protecting zinc anodes. Chinese Journal of Inorganic Chemistry, 2024, 40(7): 1243-1253. doi: 10.11862/CJIC.20240110
17. [17]
  Jianyu Qin , Yuejiao An , Yanfeng Zhang . In Situ Assembled ZnWO₄/g-C₃N₄ S-Scheme Heterojunction with Nitrogen Defect for CO₂ Photoreduction. Acta Physico-Chimica Sinica, 2024, 40(12): 2408002-. doi: 10.3866/PKU.WHXB202408002
18. [18]
  .
  南开大学师唯/华北电力大学（保定）刘景维：二维配位聚合物中有序的亲锂冠醚位点用于无枝晶锂沉积
  . CCS Chemistry, 2025, 7(0): -.
19. [19]
  Shipeng WANG , Shangyu XIE , Luxian LIANG , Xuehong WANG , Jie WEI , Deqiang WANG . Piezoelectric effect of Mn, Bi co-doped sodium niobate for promoting cell proliferation and bacteriostasis. Chinese Journal of Inorganic Chemistry, 2024, 40(10): 1919-1931. doi: 10.11862/CJIC.20240094
20. [20]
  Lijuan Wang , Yuping Ning , Jian Li , Sha Luo , Xiongfei Luo , Ruiwen Wang . Enhancing the Advanced Nature of Natural Product Chemistry Laboratory Courses with New Research Findings: A Case Study of the Application of Berberine Hydrochloride in Photodynamic Antimicrobial Films. University Chemistry, 2024, 39(11): 241-250. doi: 10.12461/PKU.DXHX202403017

Get Citation

PDF

XML

Metrics

PDF Downloads(99)
Abstract views(503)
HTML views(24)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142

Effect of Lauryl Sodium Sulfate on the In situ Crystallization of Small-Grain NaY

南开大学师唯/华北电力大学（保定）刘景维：二维配位聚合物中有序的亲锂冠醚位点用于无枝晶锂沉积

Metrics

通讯作者: 陈斌, bchen63@163.com