Citation: ZHANG Xiang-Xiong, CHEN Min. Influence of Homogeneous Electric Field on the Structure and Growth of Ice[J]. Acta Physico-Chimica Sinica, ;2014, 30(7): 1208-1214. doi: 10.3866/PKU.WHXB201405095 shu

Influence of Homogeneous Electric Field on the Structure and Growth of Ice

1.
Department of Engineering Mechanics, Tsinghua University, Beijing 100084, P. R. China

Received Date: 14 March 2014
Available Online: 9 May 2014
Fund Project:

Homogeneous crystallization of supercooled water under electric field with strength ranging from 4.0 to 40.0 V·nm^-1 was investigated by using molecular simulation technique. The liquid-solid transition was successfully obtained based on ice component analysis using the CHILL al rithm. The analysis suggested that the produced crystalline was cubic ice dominant. The influence of the field strength on the structure and the growth rate of the ice was studied. The results revealed that the presence of an electric field drove the system to crystallize rapidly into dense and distorted cubic ice. The density of the crystals increased as a function of the field strength, from 0.98 to 1.08 g·cm^-3. The growth rate of the ice nucleus increased along with the field strength according to the characteristic time derived from the Avrami equation which ranged from 0.254 to 5.513 ns. This type of acceleration can be partially attributed to the enhancement of the rotational dynamics of the water molecules. Moreover, by monitoring the formation history of the cubic ice, we found that the defective ice acted as a transition state linking the liquid water and the cubic ice.
- Molecular dynamics simulation,
- Homogeneous electric field,
- Ice crystal structure,
- Growth rate of ice crystal,
- Defective ice molecule
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