Citation:
HUANG Bo, SUN Xian-Zhong, ZHANG Xiong, ZHANG Da-Cheng, MA Yan-Wei. Organic Electrolytes for Activated Carbon-Based Supercapacitors with Flexible Package[J]. Acta Physico-Chimica Sinica,
;2013, 29(09): 1998-2004.
doi:
10.3866/PKU.WHXB201307031
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We fabricated activated carbon (AC)-based supercapacitors encased in flexible packaging using a novel organic electrolyte, triethylmethylammonium tetrafluoroborate/acetonitrile+propylene carbonate (MeEt3NBF4/(AN+PC)), and two conventional organic electrolytes, tetraethylammonium tetrafluoroborate/acetonitrile (Et4NBF4/AN) and tetraethylammonium tetrafluoroborate/propylene carbonate (Et4NBF4/PC). Cyclic voltammetry and electrochemical impedance spectroscopy measurements in various voltage windows were conducted. In addition, a comprehensive comparison of these three electrolytes was conducted via data obtained from cyclic voltammetry, electrochemical impedance spectroscopy, galvanostatic charge-discharge, leakage current, self-discharge, cyclic life, and coulombic efficiency within the 0-3 V voltage window. The results indicate that MeEt3NBF4/(AN+PC) combining the advantages of AN and PC exhibits excellent performance.
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Keywords:
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Supercapacitor
, - Organic electrolyte,
- Activated carbon
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