Citation: XIA Da-Hai, SONG Shi-Zhe, WANG Ji-Hui, BI Hui-Chao, HAN Zhe-Wen. Corrosion Behavior of Tinplates in a Functional Beverage[J]. Acta Physico-Chimica Sinica, ;2012, 28(01): 121-126. doi: 10.3866/PKU.WHXB201228121 shu

Corrosion Behavior of Tinplates in a Functional Beverage

1.
1. School of Materials Science and Engineering, Tianjin University, Tianjin 300072, P. R. China;
2. Tianjin Key Laboratory of Composite and Functional Materials, Tianjin 300072, P. R. China

Received Date: 29 September 2011
Available Online: 28 October 2011
Fund Project: 国家重点基础研究发展规划项目(973) (2011CB610500)资助 (973) (2011CB610500)

In this paper, the corrosion process of a tinplate in a functional beverage was investigated using electrochemical impedance spectroscope (EIS), scanning electron microscopy (SEM), energy dispersive X-ray spectroscopy (EDS), scanning probe microscopy (SPM), and X-ray photoelectron spectroscopy (XPS), and a corrosion mechanism is proposed. We conclude that an increase in the impedance modulus at low frequency is due to the corrosion product forming on the surface of the tinplate over the first 31 h. With an increase in the immersion time a decrease in the impedance modulus at low frequency is due to the detachment of the corrosion product and the corrosion of the carbon steel substrate. X-ray photoelectron spectroscopy (XPS) results show that the corrosion product is mainly composed of a Sn(II)/Sn(IV) citrate complex or an Fe(III) citrate complex. Furthermore, the corrosion product film is first enriched with Sn and then enriched with Fe after immersion in functional beverage for 24 d. We propose that the tinplate is mainly corroded by the organic acids that exist in functional beverages.
- Tinplate,
- Functional beverage,
- Corrosion mechanism,
- Electrochemical impedance spectroscope,
- X-ray photoelectron spectroscopy,
- Scanning probe microscopy
1. [1]
  (1) Huang, X. Q.; Li, N.; Cao, L. X.; Zheng, H. Mater. Lett. 2008,62, 466.
2. [2]
  (2) Xia, D.;Wang, J.; Song, S.; Zhong, B.; Han, Z. Advanced Materials Research 2011, 233 -235, 1747.
3. [3]
  (3) Toniolo, R.; Pizzariello, A.; Tubaro, F.; Susmel, S.; Dossi, N.;Bontempelli, G. J. Appl. Electrochem. 2009, 39, 979.
4. [4]
  (4) Patrick, G.W. Anti-Corros. Method. M. 1976, 23 (6), 9.
5. [5]
  (5) Blunden, S.;Wallace, T. Food Chem. Toxicol. 2003, 41, 1651.
6. [6]
  (6) Boogaard, P. J.; Boisset, M.; Blunden, S.; Davies, S.; Ong, T. J.;Taverne, J. P. Food Chem. Toxicol. 2003, 41, 1663.
7. [7]
  (7) Huang, B. X.; Tornatore, P.; Li, Y. S. Electrochim. Acta 2000,46, 671.
8. [8]
  (8) Sasaki, T.; Kanagawa, R.; Ohtsuka, T.; Miura, K. Corrosion Sci.2003, 45, 847.
9. [9]
  (9) Tselesh, A.S. Thin Solid Films 2008, 516, 1037.
10. [10]
  (10) Refaey, S. A. M.; Schwitzgebel, G. Appl. Surf. Sci. 1998, 135
11. [11]
  (1-4), 243.
12. [12]
  (11) Jafarian, M.; bal, F.; Danaee, I.; Biabani, R.; Mahjani, M. G.Electrochim. Acta 2008, 53, 4528.
13. [13]
  (12) El-Sherbini, E. E. F.; Abd-El-Wahab, S. M.; Amin, M. A.;Deyab, M. A. Corrosion Sci. 2006, 48, 1885.
14. [14]
  (13) Almeida, C. M. V. B.; Giannetti, B. F. Mater. Chem. Phys. 2001,69 (1-3), 261.
15. [15]
  (14) Gervasi, C. A.; Palacios, P. A.; Bimbi, M. V. F.; Alvarez, P. E.J. Electroanal. Chem. 2010, 639 (1-2), 141.
16. [16]
  (15) Zumelzua, E.; Cabezasb, C. Mater. Charact. 1995, 34, 143.
17. [17]
  (16) Kontominas, M. G.; Prodromidis, M. I.; Paleolo s, E. K.;Badeka, A. V.; Georgantelis, D. Food Chem. 2006, 98, 225.
18. [18]
  (17) Haanappel, V. A. C.; Stroosnijder, M. F. Corrosion 2001, 57,557.
19. [19]
  (18) Doherty, M.; Sykes, J. M. Corrosion Sci. 2008, 50, 2755.
20. [20]
  (19) Liu, X.; Xiong, J.; Lv, Y.; Zuo, Y. Prog. Org. Coat. 2009, 64,497.
21. [21]
  (20) Zhang,W.;Wang, J.; Zhao, Z. Y.; Jiang, J. Chem. J. Chin. Univ.2009, 30, 762. [张伟, 王佳, 赵增元, 姜晶. 高等学校化学学报, 2009, 30, 762.]
22. [22]
  (21) Rezaei, F.; Sharif, F.; Sarabi, A. A.; Kasiriha, S. M.; Rahmanian,M.; Akbarinezhad, E. J. Coat. Technol. Res. 2010, 7, 209.
23. [23]
  (22) Zhu, Y. F.; Xiong, J. P.; Tang, Y. M.; Zuo, Y. Prog. Org. Coat.2010, 69, 7.
24. [24]
  (23) Betova, I.; Bojinov, M.; Karastoyanov, V.; Kinnunen, P.; Saario,T. Electrochim. Acta 2010, 55, 6163.
25. [25]
  (24) Huang, X. Q.; Li, N.;Wang, H. Y.; Sun, H. X.; Sun, S. S.;Zheng, H. Thin Solid Films 2008, 516, 1037.
26. [26]
  (25) Graat, P. C. J.; Somers, M. A. J. Appl. Surf. Sci. 1996, 100-101,36.
27. [27]
  (26) Abd El Rehim, S. S.; Hassan, H. H.; Mohamed, N. F. Corrosion Sci. 2004, 46, 1071.
1. [1]
  Yong Zhou , Jia Guo , Yun Xiong , Luying He , Hui Li . Comprehensive Teaching Experiment on Electrochemical Corrosion in Galvanic Cell for Chemical Safety and Environmental Protection Course. University Chemistry, 2024, 39(7): 330-336. doi: 10.3866/PKU.DXHX202310109
2. [2]
  Tiantian MA , Sumei LI , Chengyu ZHANG , Lu XU , Yiyan BAI , Yunlong FU , Wenjuan JI , Haiying YANG . Methyl-functionalized Cd-based metal-organic framework for highly sensitive electrochemical sensing of dopamine. Chinese Journal of Inorganic Chemistry, 2024, 40(4): 725-735. doi: 10.11862/CJIC.20230351
3. [3]
  Li Jiang , Changzheng Chen , Yang Su , Hao Song , Yanmao Dong , Yan Yuan , Li Li . Electrochemical Synthesis of Polyaniline and Its Anticorrosive Application: Improvement and Innovative Design of the “Chemical Synthesis of Polyaniline” Experiment. University Chemistry, 2024, 39(3): 336-344. doi: 10.3866/PKU.DXHX202309002
4. [4]
  Yongming Zhu , Huili Hu , Yuanchun Yu , Xudong Li , Peng Gao . Construction and Practice on New Form Stereoscopic Textbook of Electrochemistry for Energy Storage Science and Engineering: Taking Basic Course of Electrochemistry as an Example. University Chemistry, 2024, 39(8): 44-47. doi: 10.3866/PKU.DXHX202312086
5. [5]
  Jinfu Ma , Hui Lu , Jiandong Wu , Zhongli Zou . Teaching Design of Electrochemical Principles Course Based on “Cognitive Laws”: Kinetics of Electron Transfer Steps. University Chemistry, 2024, 39(3): 174-177. doi: 10.3866/PKU.DXHX202309052
6. [6]
  Xuan Zhou , Yi Fan , Zhuoqi Jiang , Zhipeng Li , Guowen Yuan , Laiying Zhang , Xu Hou . Liquid Gating Mechanism and Basic Properties Characterization: a New Experimental Design for Interface and Surface Properties in the Chemistry “101 Plan”. University Chemistry, 2024, 39(10): 113-120. doi: 10.12461/PKU.DXHX202407111
7. [7]
  Linbao Zhang , Weisi Guo , Shuwen Wang , Ran Song , Ming Li . Electrochemical Oxidation of Sulfides to Sulfoxides. University Chemistry, 2024, 39(11): 204-209. doi: 10.3866/PKU.DXHX202401009
8. [8]
  Hao Wu , Zhen Liu , Dachang Bai . ¹H NMR Spectrum of Amide Compounds. University Chemistry, 2024, 39(3): 231-238. doi: 10.3866/PKU.DXHX202309020
9. [9]
  Wei Li , Guoqiang Feng , Ze Chang . Teaching Reform of X-ray Diffraction Using Synchrotron Radiation in Materials Chemistry. University Chemistry, 2024, 39(3): 29-35. doi: 10.3866/PKU.DXHX202308060
10. [10]
  Liangzhen Hu , Li Ni , Ziyi Liu , Xiaohui Zhang , Bo Qin , Yan Xiong . A Green Chemistry Experiment on Electrochemical Synthesis of Benzophenone. University Chemistry, 2024, 39(6): 350-356. doi: 10.3866/PKU.DXHX202312001
11. [11]
  Jinyao Du , Xingchao Zang , Ningning Xu , Yongjun Liu , Weisi Guo . Electrochemical Thiocyanation of 4-Bromoethylbenzene. University Chemistry, 2024, 39(6): 312-317. doi: 10.3866/PKU.DXHX202310039
12. [12]
  Zhengli Hu , Jia Wang , Yi-Lun Ying , Shaochuang Liu , Hui Ma , Wenwei Zhang , Jianrong Zhang , Yi-Tao Long . Exploration of Ideological and Political Elements in the Development History of Nanopore Electrochemistry. University Chemistry, 2024, 39(8): 344-350. doi: 10.3866/PKU.DXHX202401072
13. [13]
  Cunming Yu , Dongliang Tian , Jing Chen , Qinglin Yang , Kesong Liu , Lei Jiang . Chemistry “101 Program” Synthetic Chemistry Experiment Course Construction: Synthesis and Properties of Bioinspired Superhydrophobic Functional Materials. University Chemistry, 2024, 39(10): 101-106. doi: 10.12461/PKU.DXHX202408008
14. [14]
  Yajun Jian , Quanguo Zhai , Quan Gu , Shengli Gao . Reconstruction and Practice of the Teaching Content of “Carbon Group Elements” in Inorganic Chemistry to Reflect Comprehensive Education Function. University Chemistry, 2024, 39(11): 96-107. doi: 10.12461/PKU.DXHX202403006
15. [15]
  Jiahong ZHENG , Jiajun SHEN , Xin BAI . Preparation and electrochemical properties of nickel foam loaded NiMoO₄/NiMoS₄ composites. Chinese Journal of Inorganic Chemistry, 2024, 40(3): 581-590. doi: 10.11862/CJIC.20230253
16. [16]
  Zhihuan XU , Qing KANG , Yuzhen LONG , Qian YUAN , Cidong LIU , Xin LI , Genghuai TANG , Yuqing LIAO . Effect of graphene oxide concentration on the electrochemical properties of reduced graphene oxide/ZnS. Chinese Journal of Inorganic Chemistry, 2024, 40(7): 1329-1336. doi: 10.11862/CJIC.20230447
17. [17]
  Qin ZHU , Jiao MA , Zhihui QIAN , Yuxu LUO , Yujiao GUO , Mingwu XIANG , Xiaofang LIU , Ping NING , Junming GUO . Morphological evolution and electrochemical properties of cathode material LiAl_0.08Mn_1.92O₄ single crystal particles. Chinese Journal of Inorganic Chemistry, 2024, 40(8): 1549-1562. doi: 10.11862/CJIC.20240022
18. [18]
  Qingtang ZHANG , Xiaoyu WU , Zheng WANG , Xiaomei WANG . Performance of nano Li₂FeSiO₄/C cathode material co-doped by potassium and chlorine ions. Chinese Journal of Inorganic Chemistry, 2024, 40(9): 1689-1696. doi: 10.11862/CJIC.20240115
19. [19]
  Kun Xu , Xinxin Song , Zhilei Yin , Jian Yang , Qisheng Song . Comprehensive Experimental Design of Preferential Orientation of Zinc Metal by Heat Treatment for Enhanced Electrochemical Performance. University Chemistry, 2024, 39(4): 192-197. doi: 10.3866/PKU.DXHX202309050
20. [20]
  Zhonghua Xi , Xuanfeng Kong , Jinyue Yang , Bin Liu , Tingyu Zhu , Hui Zhang , Wenwei Zhang . Construction of Public Teaching Instrument Platform and Exploration of Opening Mechanism. University Chemistry, 2024, 39(7): 200-206. doi: 10.12461/PKU.DXHX202405123

Get Citation

PDF

XML

Metrics

PDF Downloads(792)
Abstract views(2459)
HTML views(11)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142