Citation:
LIU Ben-Kang, WANG Yan-Qiu, WANG Li. Time-Resolved Multiphoton Ionization Process of Xenon Investigated by Photoelectron Imaging Method[J]. Acta Physico-Chimica Sinica,
;2010, 26(12): 3157-3162.
doi:
10.3866/PKU.WHXB20101220
-
Femtosecond time-resolved multiphoton ionization dynamics of xenon was investigated using a homemade ion imaging detector. A comparison experiment comprising of the multiphoton ionization of Xe at 408 nm showed that the energy resolution of our homemade image detector was similar to that of a commercial detector. Under 272 nm femtosecond laser irradiation, photoelectrons with a kinetic energy of 1.57 and 0.26 eV, produced by three-photon ionization, corresponded to two different Xe + spin states, respectively. For the ionization at 408 nm, an additional first-order above-threshold ionization of Xe was also observed. In the two-color femtosecond time-resolved experiments, the photoelectron kinetic energy spectra varied with the delay time between the pump and the probe. The photoelectron intensities produced by 3+1' and 4'+1 two-color multiphoton ionization schedules became stronger with an increase in the degree of overlap between the two laser beams. The kinetic energy of the photoelectrons produced by one-color multiphoton ionization showed obvious red shifts, which were modulated by the second laser beam. Depopulation of the excited states was also observed upon application of the second laser beam. The red shifts in the photoelectron kinetic energy spectra reflect the time-dependent dynamical modulation process of the laser induced ponderomotive effect in an atomic system.
-
-
-
[1]
1. Bordas, C.; Dyer, M. J.; Fairfield, T.; Helm, H.; Kulander, K. C. Phys. Rev. A, 1995, 51: 3726
-
[2]
2. Schyja, V.; Lang, T.; Helm, H. Phys. Rev. A, 1998, 57: 3692
-
[3]
3. Wiehle, R.;Witzel, B. Phys. Rev. Lett., 2002, 89: 223002
-
[4]
4. A stini, P.; Breger, P.; L' Huillier, A.; Muller, H. G.; Petite, G. Phys. Rev. Lett., 1989, 63: 2208
-
[5]
5. Vrijen, R. B.; Hoogenraad, J. H.; Muller, H. G.; Noordam, L. D. Phys. Rev. Lett., 1993, 70: 3016
-
[6]
6. de Boer, M. P.; Muller, H. G. J. Phys. B: At. Mol. Opt. Phys., 1994, 27: 721
-
[7]
7. Rottke, H.; Ludwig, J.; Sandner,W. J. Phys. B: At. Mol. Opt. Phys., 1996, 29: 1479
-
[8]
8. Gingras, G.; Tripathi, A.;Witzel, B. Phys. Rev. Lett., 2009, 103: 173001
-
[9]
9. Haber, L. H.; Doughty, B.; Leone, S. R. Phys. Rev. A, 2009, 79: 031401
-
[10]
10. Aron, K.; Johnson, P. M. J. Chem. Phys., 1977, 67: 5099
-
[11]
11. A stini, P.; Fabre, F.; Mainfray, G.; Petite, G.; Rahman, N. K. Phys. Rev. Lett., 1979, 42: 1127
-
[12]
12. Freeman, R. R.; Bucksbaum, P. H.; Milchberg, H.; Darack, S.; Schumacher, D.; Geusic, M. E. Phys. Rev. Lett., 1987, 59: 1092
-
[13]
13. Paulus, G. G.; Nicklich,W.; Xu, H.; Lambropoulos, P.;Walther, H. Phys. Rev. Lett., 1994, 72: 2851
-
[14]
14. Hansch, P.;Walker, M. A.; VanWoerkom, L. D. Phys. Rev. A, 1997, 55: R2535
-
[15]
15. Hertlein, M. P.; Bucksbaum, P. H.; Muller, H. G. J. Phys. B: At. Mol. Opt. Phys., 1997, 30: L197
-
[16]
16. Böhmer, K.; Halfmann, T.; Yatsenko, L. P.; Charalambidis, C.; Horsmans, A.; Bergmann, K. Phys. Rev. A, 2002, 66: 013406
-
[17]
17. Stellpflug, M.; Johnsson, M.; Petrov, I. D.; Halfmann, T. Eur. Phys. J. D, 2003, 23: 35
-
[18]
18. Kaminski, P.;Wiehle, R.; Renard, V.; Kazmierczak, A.; Lavorel, B.; Faucher, O.;Witzel, B. Phys. Rev. A, 2004, 70: 053413
-
[19]
19. Gilb, S.; Torres, E. A.; Leone, S. R. J. Phys. B: At. Mol. Opt. Phys., 2006, 39: 4231 3161
-
[20]
20. Loh, Z. H.; Khalil, M.; Correa, R. E.; Santra, R.; Buth, C.; Leone, S. R. Phys. Rev. Lett., 2007, 98: 143601
-
[21]
21. Solomon, J. J. Chem. Phys., 1967, 47: 889
-
[22]
22. Chandler, D.W.; Houston, P. L. J. Chem. Phys., 1987, 87: 1445
-
[23]
23. Eppink, A. T. J. B.; Parker, D. H. Rev. Sci. Instrum., 1997, 68: 3477
-
[24]
24. Smith, L. M.; Keefer, D. R.; Sudharsanan, S. I. J. Quant. Spectrosc. Radiat. Transfer., 1988, 39: 367
-
[25]
25. Bordas, C.; Paulig, F.; Helm, H.; Huestis, D. L. Rev. Sci. Instrum., 1996, 67: 2257
-
[26]
26. Zhu, J. Y.;Wang, B. X.; Guo,W.;Wang, Y. Q.;Wang, L. Chin. Phys. Lett., 2007, 24: 1922
-
[27]
27. Stolow, A.; Bragg, A. E.; Neumark, D. M. Chem. Rev., 2004, 104: 1719
-
[28]
28. Wang, B. X.; Liu, B. K.;Wang, Y. Q.;Wang, L. Phys. Rev. A, 2010, 81: 043421
-
[29]
29. Saloman, E. B. J. Phys. Chem. Ref. Data, 2004, 33: 765
-
[30]
30. A stini, P.; Kupersztych, J.; LompréL, A.; Petite, G.; Yergeau, F. Phys. Rev. A, 1987, 36: 4111
-
[31]
31. Micheal, D. P.; Landen, O. L. Phys. Rev. A, 1988, 38: 2815
-
[32]
32. Schmidt, T.W.; Lopez-Martens, R. B.; Roberts, G. J. Phys. B: At. Mol. Opt. Phys., 2004, 37: 1125
-
[33]
33. Schmitt, M.; Lochbrunner, S.; Shaffer, J. P.; Larsen, J. J.; Zgierski, M. Z.; Stolow, A. J. Chem. Phys., 2001, 114: 1206
-
[1]
-
-
-
[1]
Liang TANG , Jingfei NI , Kang XIAO , Xiangmei LIU . Synthesis and X-ray imaging application of lanthanide-organic complex-based scintillators. Chinese Journal of Inorganic Chemistry, 2024, 40(10): 1892-1902. doi: 10.11862/CJIC.20240139
-
[2]
Tongyu Zheng , Teng Li , Xiaoyu Han , Yupei Chai , Kexin Zhao , Quan Liu , Xiaohui Ji . A DIY pH Detection Agent Using Persimmon Extract for Acid-Base Discoloration Popularization Experiment. University Chemistry, 2024, 39(5): 27-36. doi: 10.3866/PKU.DXHX202309107
-
[3]
Chongjing Liu , Yujian Xia , Pengjun Zhang , Shiqiang Wei , Dengfeng Cao , Beibei Sheng , Yongheng Chu , Shuangming Chen , Li Song , Xiaosong Liu . Understanding Solid-Gas and Solid-Liquid Interfaces through Near Ambient Pressure X-Ray Photoelectron Spectroscopy. Acta Physico-Chimica Sinica, 2025, 41(2): 100013-. doi: 10.3866/PKU.WHXB202309036
-
[4]
Siyi ZHONG , Xiaowen LIN , Jiaxin LIU , Ruyi WANG , Tao LIANG , Zhengfeng DENG , Ao ZHONG , Cuiping HAN . Targeting imaging and detection of ovarian cancer cells based on fluorescent magnetic carbon dots. Chinese Journal of Inorganic Chemistry, 2024, 40(8): 1483-1490. doi: 10.11862/CJIC.20240093
-
[5]
Donghui PAN , Yuping XU , Xinyu WANG , Lizhen WANG , Junjie YAN , Dongjian SHI , Min YANG , Mingqing CHEN . Preparation and in vivo tracing of 68Ga-labeled PM2.5 mimetic particles for positron emission tomography imaging. Chinese Journal of Inorganic Chemistry, 2024, 40(4): 669-676. doi: 10.11862/CJIC.20230468
-
[6]
Li'na ZHONG , Jingling CHEN , Qinghua ZHAO . Synthesis of multi-responsive carbon quantum dots from green carbon sources for detection of iron ions and L-ascorbic acid. Chinese Journal of Inorganic Chemistry, 2025, 41(4): 709-718. doi: 10.11862/CJIC.20240280
-
[7]
Chun-Lin Sun , Yaole Jiang , Yu Chen , Rongjing Guo , Yongwen Shen , Xinping Hui , Baoxin Zhang , Xiaobo Pan . Construction, Performance Testing, and Practical Applications of a Home-Made Open Fluorescence Spectrometer. University Chemistry, 2024, 39(5): 287-295. doi: 10.3866/PKU.DXHX202311096
-
[8]
Pengcheng Yan , Peng Wang , Jing Huang , Zhao Mo , Li Xu , Yun Chen , Yu Zhang , Zhichong Qi , Hui Xu , Henan Li . Engineering Multiple Optimization Strategy on Bismuth Oxyhalide Photoactive Materials for Efficient Photoelectrochemical Applications. Acta Physico-Chimica Sinica, 2025, 41(2): 100014-. doi: 10.3866/PKU.WHXB202309047
-
[9]
Zian Lin , Yingxue Jin . Matrix-Assisted Laser Desorption/Ionization Mass Spectrometry (MALDI-MS) for Disease Marker Screening and Identification: A Comprehensive Experiment Teaching Reform in Instrumental Analysis. University Chemistry, 2024, 39(11): 327-334. doi: 10.12461/PKU.DXHX202403066
-
[10]
Xingchao Zhao , Xiaoming Li , Ming Liu , Zijin Zhao , Kaixuan Yang , Pengtian Liu , Haolan Zhang , Jintai Li , Xiaoling Ma , Qi Yao , Yanming Sun , Fujun Zhang . 倍增型全聚合物光电探测器及其在光电容积描记传感器上的应用. Acta Physico-Chimica Sinica, 2025, 41(1): 2311021-. doi: 10.3866/PKU.WHXB202311021
-
[11]
Yuhang Zhang , Weiwei Zhao , Hongwei Liu , Junpeng Lü . 基于低维材料的自供电光电探测器研究进展. Acta Physico-Chimica Sinica, 2025, 41(3): 2310004-. doi: 10.3866/PKU.WHXB202310004
-
[12]
Yao Ma , Xin Zhao , Hongxu Chen , Wei Wei , Liang Shen . Progress and Perspective of Perovskite Thin Single Crystal Photodetectors. Acta Physico-Chimica Sinica, 2025, 41(4): 100030-. doi: 10.3866/PKU.WHXB202309045
-
[13]
Jinlong YAN , Weina WU , Yuan WANG . A simple Schiff base probe for the fluorescent turn-on detection of hypochlorite and its biological imaging application. Chinese Journal of Inorganic Chemistry, 2024, 40(9): 1653-1660. doi: 10.11862/CJIC.20240154
-
[14]
Ruoxi Sun , Yiqian Xu , Shaoru Rong , Chunmiao Han , Hui Xu . The Enchanting Collision of Light and Time Magic: Exploring the Footprints of Long Afterglow Lifetime. University Chemistry, 2024, 39(5): 90-97. doi: 10.3866/PKU.DXHX202310001
-
[15]
Jinfu Ma , Hui Lu , Jiandong Wu , Zhongli Zou . Teaching Design of Electrochemical Principles Course Based on “Cognitive Laws”: Kinetics of Electron Transfer Steps. University Chemistry, 2024, 39(3): 174-177. doi: 10.3866/PKU.DXHX202309052
-
[16]
Meiqing Yang , Lu Wang , Haozi Lu , Yaocheng Yang , Song Liu . Recent Advances of Functional Nanomaterials for Screen-Printed Photoelectrochemical Biosensors. Acta Physico-Chimica Sinica, 2025, 41(2): 100018-. doi: 10.3866/PKU.WHXB202310046
-
[17]
Yonghui ZHOU , Rujun HUANG , Dongchao YAO , Aiwei ZHANG , Yuhang SUN , Zhujun CHEN , Baisong ZHU , Youxuan ZHENG . Synthesis and photoelectric properties of fluorescence materials with electron donor-acceptor structures based on quinoxaline and pyridinopyrazine, carbazole, and diphenylamine derivatives. Chinese Journal of Inorganic Chemistry, 2024, 40(4): 701-712. doi: 10.11862/CJIC.20230373
-
[18]
Hong LI , Xiaoying DING , Cihang LIU , Jinghan ZHANG , Yanying RAO . Detection of iron and copper ions based on gold nanorod etching colorimetry. Chinese Journal of Inorganic Chemistry, 2024, 40(5): 953-962. doi: 10.11862/CJIC.20230370
-
[19]
Shanghua Li , Malin Li , Xiwen Chi , Xin Yin , Zhaodi Luo , Jihong Yu . 基于高离子迁移动力学的取向ZnQ分子筛保护层实现高稳定水系锌金属负极的构筑. Acta Physico-Chimica Sinica, 2025, 41(1): 2309003-. doi: 10.3866/PKU.WHXB202309003
-
[20]
Qilong Fang , Yiqi Li , Jiangyihui Sheng , Quan Yuan , Jie Tan . Magical Pesticide Residue Detection Test Strips: Aptamer-based Lateral Flow Test Strips for Organophosphorus Pesticide Detection. University Chemistry, 2024, 39(5): 80-89. doi: 10.3866/PKU.DXHX202310004
-
[1]
Metrics
- PDF Downloads(1156)
- Abstract views(2595)
- HTML views(8)