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Citation: LIU Fu-Sheng, JI Ren, WU Min, SUN Yue-Ming. Hydrogen Production from Water Splitting Using Perylene Dye-Sensitized Pt/TiO₂ Photocatalyst[J]. Acta Physico-Chimica Sinica, ;2007, 23(12): 1899-1904. doi: 10.3866/PKU.WHXB20071213 shu

Hydrogen Production from Water Splitting Using Perylene Dye-Sensitized Pt/TiO₂ Photocatalyst

1.
School of Chemistry and Chemical Engineering, Southeast University, Nanjing 210096, P. R. China; Department of Chemistry and Materials Science, Nanjing Forestry University, Nanjing 210037, P. R. China

Received Date: 25 June 2007
Available Online: 11 October 2007

The photocatalyst (DPPBI/Pt/TiO2)was prepared using N,N’-di(4-pyridyl)-3,4,9,10-perylene tetracarboxylic acid bisimide (DPPBI) sensitized Pt/TiO2 and characterized by infrared spectroscopy(IR), UV-Vis diffuse reflectance spectroscopy (UV-Vis DRS), scanning electron microscopy(SEM), X-ray photoelectron spectroscopy(XPS), and X-ray diffraction (XRD). The results of characterizationshowedthat the crystal form of TiO2was anatase, Ptwas highly dispersed on the surface of TiO2 and DPPBI was adsorbed on the surface of Pt/TiO2 in DPPBI/Pt/TiO2. Hydrogen production from water splitting using photocatalyst (DPPBI/Pt/TiO2) was studied. It has been found that the rate of hydrogen evolution reaches 6.69 滋 mol·h-1·g-1 under visible light irradiation for 8 h with 300 W Xe-lamp cold light source when 250 mL reactive liquid contains 0.8 g·L-1 photocatalyst (0.1%DPPBI/0.4%Pt/TiO2) and 0.2 mol·L-1 KI.
- Perylene; Dye; Photocatalyst; Hydrogen production
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沈阳化工大学材料科学与工程学院沈阳 110142

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Hydrogen Production from Water Splitting Using Perylene Dye-Sensitized Pt/TiO2 Photocatalyst

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通讯作者: 陈斌, bchen63@163.com

Hydrogen Production from Water Splitting Using Perylene Dye-Sensitized Pt/TiO₂ Photocatalyst