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Citation: LI Hai-Ling, WANG Wen-Jing, KANG Guo-Hu, HUANG Jin-Zhao, XU Zheng. The Effect of Reactive Pressure to Fe:NiO_x Film as Anode Catalytic Film in Hydrogen Producing System by Solar Cell[J]. Acta Physico-Chimica Sinica, ;2006, 22(03): 330-334. doi: 10.3866/PKU.WHXB20060315 shu

The Effect of Reactive Pressure to Fe:NiO_x Film as Anode Catalytic Film in Hydrogen Producing System by Solar Cell

1.
Beijing Solar Energy Research Institute, Beijing 100083, P. R. China; Laboratory of Materials for Information Storage and Display, Institute of Optoelectronic Technology, Beijing Jiaotong University, Beijing 100044, P. R. China

Received Date: 7 September 2005
Available Online: 10 March 2006

By changing the sputtering conditions, Fe∶NiOx films with different catalytic behaviors were fabricated. With the increase of working pressure the overpotential in 100 mA•cm-2 changed from 780 mV at 1.0 Pa to 330 mV at 4.0 Pa. At the same time the Tafel slop also decreased dramatically from 71 mV•dec-1 to 53 mV•dec-1. Then by further analysis of EDX, XRD, XPS, SEM, we found that the crystallinity and the effective reactive surface area, especially the content of Ni3+, all can affect the catalytic properties. Lastly, we studied the transmittance of Fe:NiOx film in the range of visible light. But as the anode catalytic film, the transmittance of Fe:NiOx film is poor, especially with the increase of depth.
- Oxygen evolution reaction; Catalytic film; Hydrogen production; Overpotential; Magnetron sputtering
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The Effect of Reactive Pressure to Fe:NiOx Film as Anode Catalytic Film in Hydrogen Producing System by Solar Cell

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通讯作者: 陈斌, bchen63@163.com

The Effect of Reactive Pressure to Fe:NiO_x Film as Anode Catalytic Film in Hydrogen Producing System by Solar Cell