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电催化二氧化碳还原的铜基催化剂设计与反应机理研究进展

张泽坤 ,  荆晓生 ,  徐浩 ,  李兆宸 ,  延卫

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引用本文: 张泽坤, 荆晓生, 徐浩, 李兆宸, 延卫. 电催化二氧化碳还原的铜基催化剂设计与反应机理研究进展[J]. 分析化学, 2023, 51(3): 316-330. doi: 10.19756/j.issn.0253-3820.221456 shu
Citation:  ZHANG Ze-Kun,  JING Xiao-Sheng,  XU Hao,  LI Zhao-Chen,  YAN Wei. Advances in Design and Reaction Mechanism of Copper-based Catalysts for Electrocatalytic Carbon Dioxide Reduction[J]. Chinese Journal of Analytical Chemistry, 2023, 51(3): 316-330. doi: 10.19756/j.issn.0253-3820.221456 shu

电催化二氧化碳还原的铜基催化剂设计与反应机理研究进展

  • 1.

    西安交通大学环境科学与工程系, 西安 710049;

  • 2.

    浙江西安交通大学研究院, 杭州 311200;

  • 3.

    中联西北工程设计研究院有限公司, 西安 710077

    • 通讯作者: 徐浩,E-mail:xuhao@xjtu.edu.cn
  • 基金项目:

    国家自然科学基金(No.52270078)、陕西省自然科学基础研究计划(No.2021JM-012)、浙江省基础公益研究计划(No.LZY21E080003)和西安交通大学基本科研业务费(No.xjh012020037)资助。

摘要: 利用电催化技术和阴极区的还原反应将CO2转化为高能化学品是解决温室效应和实现人工碳循环的有效途径。与其它金属催化剂相比,Cu基催化剂因其能生成多碳产物而备受关注,但其缺点是对产物的选择性差。因此,近年来,研究者致力于探究Cu基催化剂在反应过程中的C-C偶联机制及影响因素,并对Cu基催化剂进行针对性的结构设计和实验合成。本文总结了Cu基电极上电催化CO2还原反应(CO2RR)的基本原理,分析了影响电催化CO2RR的关键因素(电催化反应器、pH值、压力和温度、CO2的流速与浓度),综述了针对Cu基催化剂改性的相关策略(合金化、纳米结构改性、杂原子掺杂、亲/疏水性、单原子催化剂)的研究进展,最后,展望了电催化CO2RR的Cu基催化剂领域的机遇与挑战,以期为今后开展相关研究提供有益参考。

English


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