Citation: Wen-Bo ZHAO, Ya-Lan ZHANG, Guang-Yu XU, Xiao JIA, Jin-Ping XUE. Conjugation of Disassembled Zincphthalocyanine-based Nanocomposites and the Synergistic Effect on Visible-light Photosensitive Activity[J]. Chinese Journal of Structural Chemistry, ;2021, 40(8): 1012-1022. doi: 10.14102/j.cnki.0254–5861.2011–3104 shu

Conjugation of Disassembled Zincphthalocyanine-based Nanocomposites and the Synergistic Effect on Visible-light Photosensitive Activity

National & Local Joint Biomedical Engineering Research Center on Photodynamic Technologies, College of Chemistry, Fuzhou University, Fuzhou 350116, China

Corresponding author: Xiao JIA, jiaxiao@fzu.edu.cn Jin-Ping XUE, xuejinping66@fzu.edu.cn
Received Date: 20 January 2021
Accepted Date: 8 April 2021

Fund Project: the National Health and Family Planning Commission jointly established Scientific Research Fund WKJ2016-2-14the Natural Science Foundation of Fujian Province 2017J05021

Figures(9)

In this research, a conjugated Pc-MIL-88B (Fe) nanoplatform was constructed via a condensation process between modified zinc phthalocyanine and MIL-88B (Fe) for the removal of organic pollutants. The as-prepared material was fully characterized by TEM, XPS, ICP, FTIR, UV-Vis, N₂ adsorption-desorption isotherm, etc. The results indicate that Pc-MIL-88B (Fe) preserved the topological structure of MIL-88B (Fe), and the micropores of framework could effectively prevent the aggregation of Pc in water. Meanwhile, the conjugated Pc-MIL-88B (Fe) basically maintains the singlet oxygen quantum yield of Pc, and behaves a much higher photocurrent intensity compared to NH₂-MIL-88B (Fe). Additionally, the photosensitive activity and reusability of Pc-MIL-88B (Fe) were evaluated by the degradation of methylene blue in aqueous solution under visible light irradiation, and the degradation mechanism was also investigated in detail.
- metal-organic frameworks,
- zinc phthalocyanine,
- photosensitive activity,
- synergistic effect
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