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Citation: Qianqian Tang, Longshuai Zhang, Jian-Ping Zou. High-Loading Fe Single-Atom Catalyst for 100% Selectivity of ¹O₂ Generation[J]. Chinese Journal of Structural Chemistry, ;2022, 41(8): 220800. doi: 10.14102/j.cnki.0254-5861.2022-0129 shu

High-Loading Fe Single-Atom Catalyst for 100% Selectivity of ¹O₂ Generation

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Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle, Nanchang Hangkong University, Nanchang 330063, China

Author Bio: Qianqian Tang, master degree candidate, studies at Nanchang Hangkong University. Her current research interests focus on the design and synthesis of single-atom catalysts and their applications in nano-photo/electrocatalysis
Longshuai Zhang received his Ph.D. degree at the Institute of Physics, CAS in 2019. His current research interests focus on the design and synthesis of single-atom catalysts and their applications in water pollution control and recycling, nano-photo/electrocatalysis, etc
Jianping Zou received his Ph.D. degree at Fujian Institute of Research on the Structure of Matter, CAS in 2007. His current research interests focus mainly on the synthesis and application of environmental functional materials, water pollution control and recycling, nano-photo/electrocatalysis, etc
Corresponding author: Longshuai Zhang, l_s_zhang1990@163.com Jian-Ping Zou, zjp_112@126.com
Received Date: 19 May 2022
Accepted Date: 29 May 2022
Available Online: 2 June 2022

Figures(1)

The carbon nitride supported Fe SAC (Fe₁/CN) catalyst with an Fe loading of 11.2 wt% tends to adsorb the terminal O of peroxymonosulfate (PMS) on Fe-N₄ sites. Consequently, the Fe₁/CN can efficiently activate PMS to generate singlet oxygen (¹O₂) with 100% selectivity and further boost the degradation of p-chlorophenol (4-CP).
1. [1]
  Zhang, L. S.; Jiang, X. H.; Zhong, Z. A.; Tian, L.; Sun, Q.; Cui, Y. T.; Lu, X.; Zou, J. P.; Luo, S. L. Carbon nitride supported high-loading Fe single-atom catalyst for activating of peroxymonosulfate to generate O-1(2) with 100% selectivity. Angew. Chem. Int. Ed. 2021, 60, 21751-21755.
2. [2]
  Jiang, X. H.; Zhang, L. S.; Liu, H. Y.; Wu, D. S.; Wu, F. Y.; Tian, L.; Liu, L. L.; Zou, J. P.; Luo, S. L.; Chen, B. B. Silver single atom in carbon nitride catalyst for highly efficient photocatalytic hydrogen evolution. Angew. Chem. Int. Ed. 2020, 59, 23112-23116
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