Citation: Jun-Hao TANG, Hai-Yan SUN, Wen MA, Mei-Ling FENG, Xiao-Ying HUANG. Recent Progress in Developing Crystalline Ion Exchange Materials for the Removal of Radioactive Ions[J]. Chinese Journal of Structural Chemistry, ;2020, 39(12): 2157-2171. doi: 10.14102/j.cnki.0254-5861.2011-3018 shu

Recent Progress in Developing Crystalline Ion Exchange Materials for the Removal of Radioactive Ions

Jun-Hao TANG ^{a, b} ,
Hai-Yan SUN ^{a, b} ,
Wen MA ^{a, b} ,
Mei-Ling FENG ^{a, b,,} ,
Xiao-Ying HUANG ^{a, b}

a.
State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China
b.
University of Chinese Academy of Sciences, Beijing 100049, China

Corresponding author: Mei-Ling FENG, fml@fjirsm.ac.cn
Received Date: 2 November 2020
Accepted Date: 16 November 2020

Fund Project: the National Natural Science Foundation of China 22076185the National Natural Science Foundation of China 21771183the National Natural Science Foundation of China 21373223the National Natural Science Foundation of China 21221001the National Natural Science Foundation of China 21171164the National Natural Science Foundation of China 20873149the National Natural Science Foundation of China 20771102the 973 programs 2014CB845603the 973 programs 2012CB821702the 973 programs 2006CB932904the Natural Science Foundation of Fujian Province 2020J06033the Natural Science Foundation of Fujian Province 2018J01027the Natural Science Foundation of Fujian Province 2010J01056FJIRSM & IUE Joint Research Fund RHZX-2018-005Chunmiao project of Haixi institute of Chinese Academy of Sciences CMZX-2014-001the Youth Innovation Promotion Association of Chinese Academy of Sciences 2011220

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The nuclear fuel cycle inevitably generates a large amount of radioactive waste liquid, which will pose a serious threat to the ecological environment and human health. Ion exchange method has received wide attention for its easy operation, low cost and no secondary pollution. However, the effective removal of radioactive ions from complex solutions still remains a serious challenge due to their environmental mobility and radiotoxicity. We have developed an efficient strategy to construct crystalline ion-exchange materials by inducing layered or three-dimensional microporous anionic frameworks by organic cations that can be effectively exchanged by radioactive metal ions. This type of materials can be applied effectively to the removal of radioactive ions from complex solutions and the removal mechanism has been deeply clarified by means of single crystal structure analyses, theoretical calculations, etc. This review summarizes our recent progress in the study of synthesis, structures and properties of radioactive ion removals for such type of crystalline ion-exchange materials.
- ion exchange,
- crystalline materials,
- metal chalcogenide,
- vanadate,
- MOF,
- organic amine,
- radionuclide remediation
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