Citation: Ruolin CHENG, Yue WANG, Fei YANG, Huagen LIANG, Shijian LU. Application of metal-organic frameworks (MOFs) in photocatalytic CO₂ cycloaddition reaction: A mini review[J]. Chinese Journal of Inorganic Chemistry, ;2025, 41(12): 2429-2440. doi: 10.11862/CJIC.20250242 shu

Application of metal-organic frameworks (MOFs) in photocatalytic CO₂ cycloaddition reaction: A mini review

Ruolin CHENG ^{1, 2,,} ,
Yue WANG ² ,
Fei YANG ² ,
Huagen LIANG ¹ ,
Shijian LU ^{1, 2,,}

1.
Jiangsu Key Laboratory of Coal-based Greenhouse Gas Control and Utilization, Carbon Neutrality Institute, China University of Mining and Technology, Xuzhou, Jiangsu 221008, China
2.
School of Chemical Engineering, China University of Mining and Technology, Xuzhou, Jiangsu 221116, China

Corresponding author: Ruolin CHENG, ruolin.cheng@cumt.edu.cn Shijian LU, lushijian@cumt.edu.cn
Received Date: 26 July 2025
Revised Date: 25 September 2025

Figures(4)

Photocatalytic CO₂ cycloaddition reaction presents a promising CO₂ conversion strategy to establish carbon neutrality. Among emerging catalysts, metal-organic frameworks (MOFs) have been regarded as paradigm-shifting photocatalysts for their atomic precision in active site engineering, controllable porosity, and exceptional photochemical stability under ambient conditions. However, inherent limitations persist in conventional MOFs, including restricted solar spectrum utilization, inefficient charge carrier separation, and inadequate epoxide activation ability. Recent breakthroughs address these challenges through multiple strategies: ligand engineering, dopant incorporation, and composite construction. This review systematically maps the evolutionary trajectory of MOF-based photocatalysts, providing mechanistic insights into structure-activity relationships and providing insights and directions for the design of high-performance MOF-based photocatalysts.
- CO₂ cycloaddition,
- photocatalysis,
- metal-organic frameworks,
- performance optimization,
- synergistic effect
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Application of metal-organic frameworks (MOFs) in photocatalytic CO2 cycloaddition reaction: A mini review

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Application of metal-organic frameworks (MOFs) in photocatalytic CO₂ cycloaddition reaction: A mini review