Citation: Rui GAO, Zhen-Yu WANG, Lu WANG, Peng CHEN, Sheng LIU, Zhi-Peng MA, Guang-Jie SHAO. Ni₂P Nanosheets on Graphene as Sulfur-Based Composite Cathode Material for Lithium-Sulfur Batteries[J]. Chinese Journal of Inorganic Chemistry, ;2022, 38(4): 685-694. doi: 10.11862/CJIC.2022.070 shu

Ni₂P Nanosheets on Graphene as Sulfur-Based Composite Cathode Material for Lithium-Sulfur Batteries

Rui GAO ^{1, 2} ,
Zhen-Yu WANG ² ,
Lu WANG ² ,
Peng CHEN ² ,
Sheng LIU ^2,, ,
Zhi-Peng MA ¹ ,
Guang-Jie SHAO ^1,,

1.
College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, Hebei 066004, China
2.
School of Materials Science and Engineering, Nankai University, Tianjin 300350, China

Corresponding author: Sheng LIU, shengliu@nankai.edu.cn Guang-Jie SHAO, shaogj@ysu.edu.cn
Received Date: 17 November 2021
Revised Date: 7 February 2022

Figures(5)

In this work, nickel phosphide (Ni₂P) nanosheets were dispersed uniformly on graphene (G) to fabricate the Ni₂P/G composite. Furthermore, the S/Ni₂P/G sulfur-based composite was prepared further for lithium-sulfur batteries. Due to the strong chemical absorbability and high electrocatalytic activity of Ni₂P nanosheets towards soluble polysulfides, S/Ni₂P/G composite showed superior electrochemical performance. In particular, under the condition of high sulfur content (80.3%) and low electrolyte usage (15 μL·mg^-1), S/Ni₂P/G composite delivered a high initial specific discharge capacity of 1 164.7 mAh·g^-1 and good cycling stability. In addition, due to the high tap density of 1.02 g·cm^-3, S/Ni₂P/G composite showed a high volumetric capacity of 954.0 mAh·cm^-3, almost 1.6 times of that for S/G composite.
- lithium-sulfur batteries,
- sulfur cathode,
- graphene,
- nickel phosphide
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Ni2P Nanosheets on Graphene as Sulfur-Based Composite Cathode Material for Lithium-Sulfur Batteries

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Ni₂P Nanosheets on Graphene as Sulfur-Based Composite Cathode Material for Lithium-Sulfur Batteries