Citation: Lan MA, Peng-Yuan QI, Lei MA, Shi-Yu DAI, Xiao-Chen XU, Yang LIU. Effect of Different Activation Energies of Crystal Growth on Luminescent Properties and Microstructure of SrZrO₃: Ce[J]. Chinese Journal of Inorganic Chemistry, ;2021, 37(6): 968-976. doi: 10.11862/CJIC.2021.123 shu

Effect of Different Activation Energies of Crystal Growth on Luminescent Properties and Microstructure of SrZrO₃: Ce

Lan MA ¹ ,
Peng-Yuan QI ^2,, ,
Lei MA ³ ,
Shi-Yu DAI ² ,
Xiao-Chen XU ² ,
Yang LIU ²

1.
Shenyang Urban Planning & Design Institute Co., Ltd., Shenyang 110004, China
2.
School of Materials Science and Engineering, Yingkou Institute of Technology, Yingkou, Liaoning 115014, China
3.
School of Materials Science and Engineering, Shenyang University of Chemical Technology, Shenyang 110142, China

Corresponding author: Peng-Yuan QI, qipengyuan@126.com
Received Date: 5 August 2020
Revised Date: 16 March 2021

Figures(9)

SrZrO₃: Ce nanoparticles were prepared by reverse coprecipitation method with different precipitants. The phase, morphology, luminescence intensity and sintering densification of the samples were analyzed by X-ray diffraction (XRD), scanning electron microscopy (SEM), thermogravimetry-differential thermal analysis (TG-DTA). The thermal analysis kinetics of different precursors were discussed. The results showed that the prismatic and nearly spherical SrZrO₃: Ce particles with good dispersion were obtained by calcining the precursors prepared with single phase and multiphase precipitants at 1 000℃ for 2 h, with the particle sizes of about 80 and 60 nm, respectively. Using Doyle Ozawa integral method and Kissinger differential method, the average apparent activation energies in different reaction stages of precursors prepared with single phase and multiphase precipitants were 94.18, 69.39, 255.72 kJ·mol^-1 and 90.46, 51.03, 232.35 kJ·mol^-1, respectively. The activation energies of crystal growth: E_{single phase}=27.97 kJ·mol^-1 and E_multiphase=22.53 kJ·mol^-1, respectively. The apparent activation energy and grain growth activation energy of the latter were lower than those of the former, which indicates that the sample prepared with multiphase precipitant reduces the synthesis energy and improves the particle activity, and its luminous intensity was obviously better than that of the sample prepared with single phase precipitant. After vacuum sintering at 1 760℃ for 4 h, the sample prepared with multiphase precipitant had uniform grain size and achieved densification.
- coprecipitation method,
- SrZrO₃: Ce particles,
- synthesis kinetics,
- activation energy,
- luminescent properties,
- microstructure
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通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142

Effect of Different Activation Energies of Crystal Growth on Luminescent Properties and Microstructure of SrZrO3: Ce

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通讯作者: 陈斌, bchen63@163.com

Effect of Different Activation Energies of Crystal Growth on Luminescent Properties and Microstructure of SrZrO₃: Ce