Citation: WANG Bin, WANG Xiao-Hong, LIU Zhe-Lin, DONG Zhe, WANG Xiao-Hui, UAN Li-Mei, XU Liang, LIU Zong-Rui. Photocatalytic Degradation Activity of Methyl Orange by Composite Catalysts of Surfantant@Polyoxoanions Weakley Type[J]. Chinese Journal of Inorganic Chemistry, ;2020, 36(10): 1865-1872. doi: 10.11862/CJIC.2020.220 shu

Photocatalytic Degradation Activity of Methyl Orange by Composite Catalysts of Surfantant@Polyoxoanions Weakley Type

WANG Bin ^1,2,, ,
WANG Xiao-Hong ¹ ,
LIU Zhe-Lin ³ ,
DONG Zhe ¹ ,
WANG Xiao-Hui ¹ ,
UAN Li-Mei ¹ ,
XU Liang ^1,2 ,
LIU Zong-Rui ^1,,

1.
College of Chemistry and Materials Science, Inner Mongolia University for the Nationalities, Tongliao, Inner Mongolia 028043, China
2.
Key Laboratory of the Natural Products Chemistry and Functional Molecular Synthesis of Autonomous Region, Tongliao, Inner Mongolia 028000, China
3.
School of Chemistry & Environment Engineering, Changchun University of Science and Technology, Changchun 130022, China

Corresponding author: WANG Bin, jluwangbin09@163.com LIU Zong-Rui, liuzr716@163.com
Received Date: 14 March 2020
Revised Date: 22 July 2020

Figures(11)

A series of complexes of surfactant@polyoxoanions were prepared by water/chloroform two-phase electrostatic encapsulating technology, employing polyoxoanion CeW₁₀O₃₆^9- with high photocatalytic activity and cationic surfactants in different structure as building blocks. The composition and structure of the complexes were analyzed by Fourier infrared spectroscopy (FTIR) and thermogravimetric analysis (TGA). The effects of various surfactants, catalyst dosage, concentration of methyl orange, and organic dyes on the photocatalytic degradation rate were investigated, in which methyl orange and surfactant@polyoxoanions complexes were used as photodegradation substrate molecule and photocatalyst, respectively. The photodegradation activities for different composite catalysts of surfac-tant@polyoxoanions are in the order of DTAB (dodecyltrimethylammonium bromide)@CeW₁₀ > TTAB (tetradecyltrimethylammonium bromide)@CeW₁₀ > CTAB (cetyltrimethylammonium bromide)@CeW₁₀ > OTAB (octadecyl trimethyl ammonium bromide)@CeW₁₀ > DODA (dioctadecyl dimethyl ammonium bromide)@CeW₁₀.
- polyoxometalates,
- composite catalyst,
- photocatalytic degradation,
- organic dye
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