Citation: CHEN Qi, XU Bing-Jie, XU Bao-Song, LIU Peng-Fei, HAN Zhao, QIU Ben. Effects of Hydroxyl Groups on Dispersibility of Silicon Nitride Powder in Aqueous Media[J]. Chinese Journal of Inorganic Chemistry, ;2018, 34(11): 2073-2080. doi: 10.11862/CJIC.2018.244 shu

Effects of Hydroxyl Groups on Dispersibility of Silicon Nitride Powder in Aqueous Media

CHEN Qi ¹ ,
XU Bing-Jie ¹ ,
XU Bao-Song ¹ ,
LIU Peng-Fei ¹ ,
HAN Zhao ^1,2,, ,
QIU Ben ¹

1.
School of Metallurgical Engineering, Anhui University of Technology, Ma'anshan, Anhui 243002, China
2.
Key Laboratory of Metallurgical Emission Reduction & Resources Recycling, Ministry of Education, Ma'anshan, Anhui 243002, China

Corresponding author: HAN Zhao, authanzhao@foxmail.com
Received Date: 4 July 2018
Revised Date: 10 August 2018

Figures(9)

The surface of silicon nitride (Si₃N₄) powder was efficiently hydroxylated via application of nitric acid to improve dispersibility in aqueous media.Hydroxylated powder results in more stable colloidal dispersion in aqueous media compared to native powder.Results of Fourier transform infrared spectroscopy and X-ray photoelectron spectroscopy show that hydroxyl group content of Si₃N₄ powder significantly increased with hydroxyl modification.This is helpful in preventing Si₃N₄ powder from aggregating in aqueous media.In addition, thermogravimetric analysis indicates that hydroxyl group content of hydroxylated Si₃N₄ powder was 68.8% higher than that of native powder.Furthermore, surface hydrophilicity of Si₃N₄ powder is enhanced with hydroxyl modification, and powder dispersibility is improved with an increase in hydroxyl content.
- silicon nitride,
- hydroxylation,
- surface modification,
- dispersibility
1. [1]
  Yusup L, Park J, Mayangsari T, et al. Appl. Surf. Sci., 2018, 1:127-131
2. [2]
  ?zcan S, A??kbas G, ?zbay N, et al. Ceram. Int., 2017, 1:10057-10065
3. [3]
  Tshabalala L, Pityana S. Surf. Coat. Technol., 2016, 289:52-60 doi: 10.1016/j.surfcoat.2016.01.028
4. [4]
  Selzer A, Brizé V, Voytovych R, et al. J. Eur. Ceram. Soc., 2017, 37(1):75-82 doi: 10.1016/j.jeurceramsoc.2016.07.021
5. [5]
  Li J, Liu M, Tan Y, et al. Int. J. App. Ceram. Technol., 2013, 10(1):40-44 doi: 10.1111/ijac.2012.10.issue-1
6. [6]
  Rueschhoff L, Trice R, Youngblood J. Ceram. Int., 2017, 43(14):10791-10798 doi: 10.1016/j.ceramint.2017.05.097
7. [7]
  Yao S L, Lin X P, Ma J T, et al. Key Eng. Mater., 2012, 512-515:837-840 doi: 10.4028/www.scientific.net/KEM.512-515
8. [8]
  Zhuang Y, Lin T, Wang S, et al. J. Eur. Ceram. Soc., 2017, 37(10):3293-3301 doi: 10.1016/j.jeurceramsoc.2017.03.031
9. [9]
  Niu F, Wang Y, Abbas I, et al. Ceram. Int., 2017, 43:3238-3245 doi: 10.1016/j.ceramint.2016.11.151
10. [10]
  Li X, Zhang L, Yin X. Scr. Mater., 2012, 67(4):380-383 doi: 10.1016/j.scriptamat.2012.05.030
11. [11]
  Schmidt D, Giannelis E. Chem. Mater., 2010, 22(1):167-174 doi: 10.1021/cm9026978
12. [12]
  Cheng G, Qian J, Tang Z, et al. Ceram. Int., 2015, 41:1789-1884
13. [13]
  Wei Q, Qian J, Miao J, et al. J. Dispersion Sci. Technol., 2012, 33(9):1385-1392 doi: 10.1080/01932691.2011.599223
14. [14]
  Sun N, Meng X, Xiao Z. Ceram. Int., 2015, 41:13830-13835 doi: 10.1016/j.ceramint.2015.08.068
15. [15]
  Iijima M, Okamura N, Tatami J. Ind. Eng. Chem. Res., 2015, 54(51):12847-12854 doi: 10.1021/acs.iecr.5b03696
16. [16]
  Lü Zhi-Jie, ZHAO Jun, AI Xing. Journal of the Chinese Ceramic Society, 2007, 35(11):1434-1438 doi: 10.3321/j.issn:0454-5648.2007.11.005
17. [17]
  Paik U, Hackley V, Haeweon L. J. Am. Ceram. Soc., 1999, 82(4):833-840 doi: 10.1111/j.1151-2916.1999.tb01843.x
18. [18]
  Laarz E, Bergstrm L. J. Eur. Ceram. Soc., 2000, 20(4):431-440 doi: 10.1016/S0955-2219(99)00187-9
19. [19]
  REN Hong-Mei, MENG Qing-Chun, FAN Zhong-Yu, et al. Journal of China University of Petroleum:Ed. Nat. Sci., 2014, 38(5):172-177
20. [20]
  Raghavan S, Walls H, Khan S, et al. Langmuir, 2000, 16(21):7920-7930 doi: 10.1021/la991548q
21. [21]
  LIU Jun, XIONG Dang-Sheng. Journal of the Chinese Ceramic Society, 2010, 38(5):908-912
22. [22]
  Bowen P, Highfield J, Mocellin A, et al. J. Am. Ceram. Soc., 1990, 21(24):724-728
23. [23]
  Egashira M, Shimizu Y, Takatsuki S. J. Mater. Sci. Lett., 1991, 10(17):994-996 doi: 10.1007/BF00721824
24. [24]
  Barnard A, Curtiss L. Nano Lett., 2005, 5(7):1261-1266 doi: 10.1021/nl050355m
25. [25]
  Mueller R, Kammler H, Wegner K, et al. Langmuir, 2003, 19(1):160-165 doi: 10.1021/la025785w
26. [26]
  Baraton M, Chang W, Kear B. J. Phys. Chem., 1996, 100(41):16647-16652 doi: 10.1021/jp961196l
27. [27]
  Zhao Q, Chen W, Zhu Q. Nanotechnology, 2004, 15(8):958-961 doi: 10.1088/0957-4484/15/8/015
28. [28]
  Li C, Metzler D, Lai C, et al. J. Vac. Sci. Technol. A, 2016, 34(4):041307 doi: 10.1116/1.4954961
29. [29]
  Janczuk B, Zdziennicka A. J. Mater. Sci., 1994, 29(13):3559-3564 doi: 10.1007/BF00352063
30. [30]
  Mu B, Wang T, Liu P. Ind. Eng. Chem. Res., 2007, 46(10):3069-3072 doi: 10.1021/ie070252+
31. [31]
  Peschel G, Belouschek P, Muller M, et al. Colloid Polym. Sci., 1982, 260(4):444-451 doi: 10.1007/BF01448150
1. [1]
  Yu Peng , Yue Wang , Tian-Jiao Chen , Jing-Jing Chen , Jin-Ling Yang , Ting Gong , Ping Zhu . A fungal CYP from Beauveria bassiana with promiscuous steroid hydroxylation capabilities. Chinese Chemical Letters, 2024, 35(5): 108818-. doi: 10.1016/j.cclet.2023.108818
2. [2]
  Chenghao Ge , Peng Wang , Pei Yuan , Tai Wu , Rongjun Zhao , Rong Huang , Lin Xie , Yong Hua . Tuning hot carrier transfer dynamics by perovskite surface modification. Chinese Chemical Letters, 2024, 35(10): 109352-. doi: 10.1016/j.cclet.2023.109352
3. [3]
  Zhenyu Hu , Zhenchun Yang , Shiqi Zeng , Kun Wang , Lina Li , Chun Hu , Yubao Zhao . Cationic surface polarization centers on ionic carbon nitride for efficient solar-driven H₂O₂ production and pollutant abatement. Chinese Chemical Letters, 2024, 35(10): 109526-. doi: 10.1016/j.cclet.2024.109526
4. [4]
  Wenhao Yan , Shuaiya Xue , Xuerui Zhao , Wei Zhang , Jian Li . Hexagonal boron nitride based slippery liquid infused porous surface with anti-corrosion, anti-contaminant and anti-icing properties for protecting magnesium alloy. Chinese Chemical Letters, 2024, 35(4): 109224-. doi: 10.1016/j.cclet.2023.109224
5. [5]
  Peng Zhou , Ziang Jiang , Yang Li , Peng Xiao , Feixiang Wu . Sulphur-template method for facile manufacturing porous silicon electrodes with enhanced electrochemical performance. Chinese Chemical Letters, 2024, 35(8): 109467-. doi: 10.1016/j.cclet.2023.109467
6. [6]
  Yang Deng , Yitao Ouyang , Chao Han . Constriction-susceptible makes fast cycling of lithium metal in solid-state batteries: Silicon as an example. Chinese Journal of Structural Chemistry, 2024, 43(7): 100276-100276. doi: 10.1016/j.cjsc.2024.100276
7. [7]
  Wenbi Wu , Yinchu Dong , Haofan Liu , Xuebing Jiang , Li Li , Yi Zhang , Maling Gou . Modification of plasma protein for bioprinting via photopolymerization. Chinese Chemical Letters, 2024, 35(8): 109260-. doi: 10.1016/j.cclet.2023.109260
8. [8]
  Mei-Chen Liu , Qing-Song Liu , Yi-Zhou Quan , Jia-Ling Yu , Gang Wu , Xiu-Li Wang , Yu-Zhong Wang . Phosphorus-silicon-integrated electrolyte additive boosts cycling performance and safety of high-voltage lithium-ion batteries. Chinese Chemical Letters, 2024, 35(8): 109123-. doi: 10.1016/j.cclet.2023.109123
9. [9]
  Zhiwei Zhong , Yanbin Huang , Wantai Yang . A simple photochemical method for surface fluorination using perfluoroketones. Chinese Chemical Letters, 2024, 35(5): 109339-. doi: 10.1016/j.cclet.2023.109339
10. [10]
  Yukai Tong , Zhijun Wu , Bo Zhou , Min Hu , Anpei Ye . Surface tension of single suspended aerosol microdroplets. Chinese Chemical Letters, 2024, 35(4): 109062-. doi: 10.1016/j.cclet.2023.109062
11. [11]
  Yu He , Hao Jiang , Shaoxuan Yuan , Jiayi Lu , Qiang Sun . On-surface photo-induced dechlorination. Chinese Chemical Letters, 2024, 35(9): 109807-. doi: 10.1016/j.cclet.2024.109807
12. [12]
  Lijun Mao , Shuo Li , Xin Zhang , Zhan-Ting Li , Da Ma . Cucurbit[n]uril-based nanostructure construction and modification. Chinese Chemical Letters, 2024, 35(8): 109363-. doi: 10.1016/j.cclet.2023.109363
13. [13]
  Fangling Cui , Zongjie Hu , Jiayu Huang , Xiaoju Li , Ruihu Wang . MXene-based materials for separator modification of lithium-sulfur batteries. Chinese Journal of Structural Chemistry, 2024, 43(7): 100337-100337. doi: 10.1016/j.cjsc.2024.100337
14. [14]
  Qiang Zhang , Weiran Gong , Huinan Che , Bin Liu , Yanhui Ao . S doping induces to promoted spatial separation of charge carriers on carbon nitride for efficiently photocatalytic degradation of atrazine. Chinese Journal of Structural Chemistry, 2023, 42(12): 100205-100205. doi: 10.1016/j.cjsc.2023.100205
15. [15]
  Wenda WANG , Jinku MA , Yuzhu WEI , Shuaishuai MA . Waste biomass-derived carbon modified porous graphite carbon nitride heterojunction for efficient photodegradation of oxytetracycline in seawater. Chinese Journal of Inorganic Chemistry, 2024, 40(4): 809-822. doi: 10.11862/CJIC.20230353
16. [16]
  Ziruo Zhou , Wenyu Guo , Tingyu Yang , Dandan Zheng , Yuanxing Fang , Xiahui Lin , Yidong Hou , Guigang Zhang , Sibo Wang . Defect and nanostructure engineering of polymeric carbon nitride for visible-light-driven CO2 reduction. Chinese Journal of Structural Chemistry, 2024, 43(3): 100245-100245. doi: 10.1016/j.cjsc.2024.100245
17. [17]
  Fabrice Nelly Habarugira , Ducheng Yao , Wei Miao , Chengcheng Chu , Zhong Chen , Shun Mao . Synergy of sodium doping and nitrogen defects in carbon nitride for promoted photocatalytic synthesis of hydrogen peroxide. Chinese Chemical Letters, 2024, 35(8): 109886-. doi: 10.1016/j.cclet.2024.109886
18. [18]
  Qianqian Song , Yunting Zhang , Jianli Liang , Si Liu , Jian Zhu , Xingbin Yan . Boron nitride nanofibers enhanced composite PEO-based solid-state polymer electrolytes for lithium metal batteries. Chinese Chemical Letters, 2024, 35(6): 108797-. doi: 10.1016/j.cclet.2023.108797
19. [19]
  Chao-Long Chen , Rong Chen , La-Sheng Long , Lan-Sun Zheng , Xiang-Jian Kong . Anchoring heterometallic cluster on P-doped carbon nitride for efficient photocatalytic nitrogen fixation in water and air ambient. Chinese Chemical Letters, 2024, 35(4): 108795-. doi: 10.1016/j.cclet.2023.108795
20. [20]
  Wengao Zeng , Yuchen Dong , Xiaoyuan Ye , Ziying Zhang , Tuo Zhang , Xiangjiu Guan , Liejin Guo . Crystalline carbon nitride with in-plane built-in electric field accelerates carrier separation for excellent photocatalytic hydrogen evolution. Chinese Chemical Letters, 2024, 35(4): 109252-. doi: 10.1016/j.cclet.2023.109252

Get Citation

PDF

XML

Metrics

PDF Downloads(15)
Abstract views(757)
HTML views(138)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142