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Citation: ZHANG Qiu-Lin, XU Li-Si, LIU Xin, NING Ping. Effect of P123 on Structure and CO Catalytic Oxidation Performance of CuO-CeO2 Catalysts[J]. Chinese Journal of Inorganic Chemistry, ;2015, 31(8): 1555-1562. doi: 10.11862/CJIC.2015.192 shu

Effect of P123 on Structure and CO Catalytic Oxidation Performance of CuO-CeO2 Catalysts

  • 1.

    Faculty of Environmental Science and Engineering, Kunming University of Science and Technology, Kunming 650500, China

  • Corresponding author: NING Ping, 
  • Received Date: 13 March 2015
    Available Online: 25 May 2015

    Fund Project: 国家自然科学基金(No.21307047、U1137603)资助项目。 (No.21307047、U1137603)

  • A series of CuO-CeO2 (nCu:nCe=1:9, 2:8, 3:7, 4:6, 5:5, 6:4, 7:3) catalysts with different Cu/Ce molar ratios (nCu:nCe) were prepared by soft template hydrothermal method. The effect of nCu:nCe and preparation methods (soft template hydrothermal method and co-precipitation without template method) on CO catalytic oxidation performance was investigated, and the structure, reduction features and surface chemical states of the CuO-CeO2 catalysts were characterized by XRD, TEM, low temperature adsorption-desorption, temperature programmed reduction (H2-TPR) and XPS. The results show that with the increase of nCu:nCe, the CO catalytic oxidation activities of CuO-CeO2 catalysts increase firstly and then decrease. When the nCu:nCe is 5:5, the CO catalytic oxidation activity of the catalyst is more than 90% at 100℃. The large specific surface area, narrow pore structure distribution, high dispersion of active CuO species and the strong interaction between CuO and CeO2 of CuO-CeO2 catalyst prepared by soft template hydrothermal method are the main factors for its excellent CO catalytic oxidation activity.
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    1. [1]

      [1] Qin J W, Lu J F, Cao M H, et al. Nanoscale, 2010,2:2739-2743

    2. [2]

      [2] Kalamaras C M, Americanou S, Efstathiou A M. J. Catal., 2011,279:287-300

    3. [3]

      [3] Kim J R, Myeong W J, Ihm Son-Ki. J. Catal., 2009,263:123-133

    4. [4]

      [4] Luo J Y, Meng M, Zha Y Q, et al. J. Phys. Chem. C, 2008, 112(23):8694-870

    5. [5]

      [5] Zheng X, Wang S, Zhang S, et al. Catal. Commun., 2004,5:729-732

    6. [6]

      [6] Zhu J, Zhang L, Deng Y, et al. Appl. Catal. B:Environ., 2010,96:449-457

    7. [7]

      [7] Luo M F, Song Y P, Lu J Q, et al. J. Phys. Chem. C, 2007, 111:12686-12692

    8. [8]

      [8] Skårman B, Grandjean D, Benfield R E, et al. J. Catal., 2002, 211:119-133

    9. [9]

      [9] Rao K N, Bharali P, Thrimurthulu G, et al. Catal. Commun., 2010,11:863-866

    10. [10]

      [10] Kundakovic L, Flytzani-Stephanopoulos M. Appl. Catal. A:Gen., 1998,171(1):13-29

    11. [11]

      [11] Kundakovic L, Flytzani-Stephanopoulos M. J. Catal., 1998, 179(1):203-221

    12. [12]

      [12] Xie X W, Li Y, Liu Z Q, et al. Nature, 2009,458:746-749

    13. [13]

      [13] Avgouropoulos G, Ioannides T. Appl. Catal. B:Environ., 2006,67(1/2):1-11

    14. [14]

      [14] Lee H C, Kim D H. Catal. Today, 2008,132:109-116

    15. [15]

      [15] Jung C R, Han J, Nam S W, et al. Catal. Today, 2004,93-95:183-190

    16. [16]

      [16] Zou H B, Chen S Z, Liu Z L, et al. Powder Technol., 2011, 207:238-244

    17. [17]

      [17] Wang W W, Du P P, Zou S H, et al. ACS Catal., 2015,5:2088-2099

    18. [18]

      [18] Li L, Song L, Wang H, et al. Int. J. Hydrogen Energy, 2011, 36:8839-8849

    19. [19]

      [19] Bera P, Aruna S T, Patil K C, et al. J. Catal., 1999,186(1):36-44

    20. [20]

      [20] Astudilloa J, Águilab G, Díaz F, et al. Appl. Catal. A:Gen., 2010,381:169-176

    21. [21]

      [21] Chadwick A V, Savin S L P. J. Alloys Compd., 2009,488:1-4

    22. [22]

      [22] Sedmak G, Hocevar S, Levec J. J. Catal., 2003,213(2):135-150

    23. [23]

      [23] Gu D, Jia C J, Bongard H, et al. Appl. Catal. B:Environ., 2014,152-153:11-18

    24. [24]

      [24] Tang C J, Sun J F, Yao X J, et al. Appl. Catal. B:Environ., 2014,146:201-212

    25. [25]

      [25] Pérez N C, Miró E E, Zamaro J M. Appl. Catal. B:Environ., 2013,129:416-425

    26. [26]

      [26] Zhou G L, Lan H, Song R Y, et al. RSC Adv., 2014,4:50840-50850

    27. [27]

      [27] Niu K, Shi D J, Dong W F, et al. J. Coll. Interf. Sci., 2011, 362(1):74-80

    28. [28]

      [28] Wang Z, Qu Z P, Quan X, et al. Appl. Catal. B:Environ., 2013,134-135:153-166

    29. [29]

      [29] Zou Z Q, Meng Ming, Guo L H, et al. J. Hazard. Mater., 2009,163:835-842

    30. [30]

      [30] Vidal H,Kǎspar J, Pijolat M, et al. Appl. Catal. B:Environ., 2000,27(1):49-63

    31. [31]

      [31] Morris S M, Horton J A, Jaroniec M. Microporous Mesopor. Mater., 2010,128:180-186

    32. [32]

      [32] Łamacz A, Krzto A, Djéga-Mariadassou G. Appl. Catal. B:Environ., 2013,142-143:268-277

    33. [33]

      [33] Vidal H,Kǎspar J, Pijolat M, et al. Appl. Catal. B:Environ., 2000,27(1):49-63

    34. [34]

      [34] Zeng S H, Wang Y, Liu K, et al. Int. J. Hydrogen Energy, 2012,37(16):11640-11649

    35. [35]

      [35] ZHANG Li-Ping(张丽萍), WAN Hai-Qin(万海勤), ZHU Jie (朱捷), et al. Chinese J. Inorg. Chem.(无机化学学报), 2007, 23(3):427-431

    36. [36]

      [36] Fan J, Wu X D, Wu X D, et al. Appl. Catal. B:Environ., 2008,81(1/2):38-48

    37. [37]

      [37] Zeng S H, Zhang W L, Sliwa M, et al. Int. J. Hydrogen Energy, 2013,38(9):3597-3605

    38. [38]

      [38] LI Zhi-Hong(李志红), HUANG Wei(黄伟), ZUO Zhi-Jun(左志军), et al. Chinese J. Catal.(催化学报), 2009,30(2):171-177

    39. [39]

      [39] Chen W T, Jovic V, Sun-Waterhouse D X, et al. Int. J. Hydrogen Energy, 2013,38(35):15036-15048

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