Citation: YUAN Su-Jun, ZHANG Qing-Hong, LEI Fang, XIE Jian-Jun, SHI Ying. Self Assembly TiO2 Films on the Flexible Transparent Conductive Oxide Substrates: Preparation and Photoelectrochemical Activity[J]. Chinese Journal of Inorganic Chemistry, ;2015, (6): 1099-1104. doi: 10.11862/CJIC.2015.165
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The all-nanoparticle TiO2 films were directly prepared on the flexible transparent conductive oxide substrates by the layer-by-layer (LBL) self assembly method through the crystallized TiO2. During the preparation, the polyelectrolytes were replaced and the calcination is avoided. The TiO2 used in the self assembling process included an anatase TiO2 sol and the Degussa P25. The microstructure of the self assembly films was controlled through the ultrafine TiO2 crystallites of the sol, which could improve the uniformity and density of the films. The TiO2 film was introduced to be the working electrode in a three-electrode photoelectrochemical bulk cell, and the one with the high uniformity and density showed a good photoelectrochemical property. The photocurrent responses obtained from the TiO2 electrodes prepared with the TiO2 sol were about 25% higher than that of the one prepared without the sol.
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