Citation: WENG Jun-Ying, ZHAO Wei, ZHANG Ying-Hui. Study on the Interaction Between C60 Bisadducts and Cyclic Porphyrin Dimer[J]. Chinese Journal of Inorganic Chemistry, ;2014, 30(5): 1079-1086. doi: 10.11862/CJIC.2014.173
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The interaction between cyclic porphyrin dimmer and four kinds of pyrrolidine di-functionalized C60 (bis-C60) isomers, namely trans-2, trans-3, trans-4, and e, has been studied by UV-Visible absorption spectroscopy. The introduction of pyrrolidine ring weakens the interaction between porphyrin dimer and fullerene in the order of C60 >mono-functionalized C60 >di-functionalized C60. Four kinds of bisadduct isomers were compared with each other in their interaction with porphyrin dimer, with an order of trans-2> trans-3≈trans-4> e isomer, which is attributed to different steric hindrance caused by different substitution pattern. The density functional theory calculation on the interaction geometry and absorption spectra were performed for the trans-3 bis-C60/cyclic porphyrin dimer complex.
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