Citation: Li Li, Xue Ke, Shan Wang, Zhuo Jiang, Yuzheng Guo, Chunguang Kuai. Antioxidative strategies of 2D MXenes in aqueous energy storage system[J]. Chinese Chemical Letters, ;2025, 36(5): 110423. doi: 10.1016/j.cclet.2024.110423 shu

Antioxidative strategies of 2D MXenes in aqueous energy storage system

Li Li ^a ,
Xue Ke ^b ,
Shan Wang ^c ,
Zhuo Jiang ^b ,
Yuzheng Guo ^{a, b, d, *,} ,
Chunguang Kuai ^{b, *,}

a.
The Institute of Technological Sciences, Wuhan University, Wuhan 430072, China
b.
School of Electrical Engineering and Automation, Wuhan University, Wuhan 430072, China
c.
Department of Anesthesiology, Zhongnan Hospital of Wuhan University, Wuhan 430072, China
d.
Hubei Key Laboratory of Electronic Manufacturing and Packaging Integration, Wuhan University, Wuhan 430072, China

yguo@whu.edu.cn

chunguangk@whu.edu.cn

Received Date: 1 December 2023
Revised Date: 19 July 2024
Accepted Date: 5 September 2024
Available Online: 7 September 2024

Figures(8)

As a novel two-dimensional (2D) material, MXenes are anticipated to have a significant impact on future aqueous energy storage and conversion technologies owing to their unique intrinsic laminar structure and exceptional physicochemical properties. Nevertheless, the fabrication and utilization of functional MXene-based devices face formidable challenges due to their susceptibility to oxidative degradation in aqueous solutions. This review begins with an outline of various preparation techniques for MXenes and their implications for structure and surface chemistry. Subsequently, the controversial oxidation mechanisms are discussed, followed by a summary of currently employed oxidation characterization techniques. Additionally, the factors influencing MXene oxidation are then introduced, encompassing chemical composition (types of M, X elements, layer numbers, terminations, and defects) as well as environment (atmosphere, temperature, light, potential, solution pH, free water and O₂ content). The review then shifts its focus to strategies aiming to prevent or delay MXene oxidation, thereby expanding the applicability of MXenes in complex environments. Finally, the challenges and prospects within this rapidly-growing research field are presented to promote further advancements of MXenes in aqueous storage systems.
- MXene oxidation,
- Mechanism,
- Characterization,
- Factors,
- Antioxidative strategies
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沈阳化工大学材料科学与工程学院沈阳 110142