Citation: Yuehai Zhi, Chen Gu, Huachao Ji, Kang Chen, Wenqi Gao, Jianmei Chen, Dafeng Yan. The advanced development of innovative photocatalytic coupling strategies for hydrogen production[J]. Chinese Chemical Letters, ;2025, 36(1): 110234. doi: 10.1016/j.cclet.2024.110234 shu

The advanced development of innovative photocatalytic coupling strategies for hydrogen production

Yuehai Zhi ^{a, 1} ,
Chen Gu ^{a, 1} ,
Huachao Ji ^a ,
Kang Chen ^a ,
Wenqi Gao ^b ,
Jianmei Chen ^{a, *,} ,
Dafeng Yan ^{b, *,}

a.
College of Electronic and Optical Engineering & College of Flexible Electronics (Future Technology), Nanjing 210023, China
b.
Hubei Key Laboratory for Precision Synthesis of Small Molecule Pharmaceuticals & Ministry of Education Key Laboratory for the Synthesis and Application of Organic Functional Molecules & College of Chemistry and Chemical Engineering, Hubei University, Wuhan 430062, China

chenjianmei@njupt.edu.cn

dafengyan@hubu.edu.cn

Received Date: 21 May 2024
Revised Date: 5 July 2024
Accepted Date: 10 July 2024
Available Online: 10 July 2024

Figures(8)

Photocatalytic technology harnesses solar energy to facilitate chemical transformations, presenting significant potential in energy generation and environmental remediation. However, the conventional O₂ evolution process is hindered by high reaction barriers and inefficiencies, which limit its widespread application. Therefore, exploring novel photocatalytic coupling strategies to replace water oxidation has become a key route to enhance the efficiency of H₂ production. In this review, organic pollutants removal and the valorization of organics as substitutes for water oxidation coupling strategies for photocatalytic H₂ production are comprehensively summarized. These strategies not only circumvent the high reaction barriers associated with O₂ evolution to enhance the H₂ production but also aid in the removing of organic pollutants or synthesis of value-added chemicals. We also present future research directions and underscore the significance of advanced catalyst design, in-depth analysis of reaction mechanisms, and systematic optimization strategies in realizing an efficient and sustainable photocatalytic process. This guidance is anticipated to provide theoretical and practical new insights for the future development of photocatalytic coupling reactions, fostering further explorations in the realm of renewable energy and environmental governance.
- Photocatalysis,
- Pollutants removal,
- Valorization of organics,
- Catalyst design
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沈阳化工大学材料科学与工程学院沈阳 110142