Citation: Xinyu Wu, Jianfeng Lu, Zihao Zhu, Suijun Liu, Herui Wen. Recent advances of metal-organic frameworks and MOF-derived materials based on p-block metal for the electrochemical reduction of carbon dioxide[J]. Chinese Chemical Letters, ;2025, 36(7): 110151. doi: 10.1016/j.cclet.2024.110151 shu

Recent advances of metal-organic frameworks and MOF-derived materials based on p-block metal for the electrochemical reduction of carbon dioxide

Xinyu Wu ^a ,
Jianfeng Lu ^a ,
Zihao Zhu ^{a, b, c, *,} ,
Suijun Liu ^{a, *,} ,
Herui Wen ^a

a.
School of Chemistry and Chemical Engineering, Jiangxi Province Key Laboratory of Functional Crystalline Materials Chemistry, Jiangxi University of Science and Technology, Ganzhou 341000, China
b.
Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education), Nankai University, Tianjin 300071, China
c.
China Tin Grp Co., Ltd., Liuzhou 545000, China

zhuzihao@jxust.edu.cn

sjliu@jxust.edu.cn

Received Date: 28 April 2024
Revised Date: 28 May 2024
Accepted Date: 20 June 2024
Available Online: 21 June 2024

Figures(23)

In recent years, reducing carbon emissions to achieve carbon neutrality has become an urgent issue for environmental protection and sustainable development. Converting CO₂ into valuable chemical products through electrocatalysis powered by renewable electricity exhibits great potential. However, the electro-reduction of CO₂ heavily relies on efficient catalysts to overcome the required energy barrier due to the high stability of CO₂. p-block metal-based MOFs and MOF-derived catalysts have been proven to be efficient catalysts for electrochemical CO₂ reduction reaction (CO₂RR) due to their unique electronic structure and clear active sites. However, factors such as conductivity and stability limit the practical application of p-block metal-based MOFs and MOF-derived catalysts. In this review, we summarize the latest progress of MOFs and MOF-derived catalysts based on typical p-block metals in the field of CO₂RR. Then the modification strategies for MOFs-based catalysts and the related catalytic mechanism are briefly introduced. Furthermore, we offer the challenges and prospects of p-block metal-based MOFs and MOF-derived catalysts in the hope of providing guidance for potential applications.
- CO₂ reduction,
- Electrocatalysis,
- p-block metal,
- Metal-organic frameworks,
- MOF-derived materials
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