Citation: Ming-Yi Sun, Lu Zhang, Ya Li, Chong-Chen Wang, Peng Wang, Xueying Ren, Xiao-Hong Yi. Recovering Ag⁺ with nano-MOF-303 to form Ag/AgCl/MOF-303 photocatalyst: The role of stored Cl⁻ ions[J]. Chinese Chemical Letters, ;2025, 36(2): 110035. doi: 10.1016/j.cclet.2024.110035 shu

Recovering Ag⁺ with nano-MOF-303 to form Ag/AgCl/MOF-303 photocatalyst: The role of stored Cl⁻ ions

Beijing Key Laboratory of Functional Materials for Building Structure and Environment Remediation, School of Environment and Energy Engineering, Beijing University of Civil Engineering and Architecture, Beijing 100044, China

wangchongchen@bucea.edu.cn

Received Date: 5 February 2024
Revised Date: 25 April 2024
Accepted Date: 20 May 2024
Available Online: 21 May 2024

Figures(6)

The nano-MOF-303 synthesized by microwave method exhibited efficient adsorption capacity (232 mg/g) toward Ag⁺, in which the adsorption behaviors were fitted by the pseudo-second-order kinetic and the Freundlich isotherm model. The outstanding Ag⁺ sorption ability of nano-MOF-303 could be contributed to electrostatic interactions, weak coordination interaction of Ag-N, and AgCl precipitates originating from the stored Cl⁻ in nano-MOF-303. Besides the adsorbent regeneration, the formed Ag/AgCl onto nano-MOF-303 could produce Ag/AgCl/MOF-303 as a photocatalyst for sulfamethoxazole degradation under visible light. In this work, both the adsorption and photocatalysis mechanisms were clarified, which might provide insight to develop more effective adsorbents for mining the critical resource from the wastewater.
- MOF-303,
- Silver ions,
- Resource recovery,
- Photocatalyst,
- Mechanism
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Recovering Ag+ with nano-MOF-303 to form Ag/AgCl/MOF-303 photocatalyst: The role of stored Cl− ions

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通讯作者: 陈斌, bchen63@163.com

Recovering Ag⁺ with nano-MOF-303 to form Ag/AgCl/MOF-303 photocatalyst: The role of stored Cl⁻ ions