Citation: Manyu Zhu, Fei Liang, Lie Wu, Zihao Li, Chen Wang, Shule Liu, Xiue Jiang. Revealing the difference of Stark tuning rate between interface and bulk by surface-enhanced infrared absorption spectroscopy[J]. Chinese Chemical Letters, ;2025, 36(2): 109962. doi: 10.1016/j.cclet.2024.109962 shu

Revealing the difference of Stark tuning rate between interface and bulk by surface-enhanced infrared absorption spectroscopy

Manyu Zhu ^{a, b, 1} ,
Fei Liang ^{c, 1} ,
Lie Wu ^a ,
Zihao Li ^{a, b} ,
Chen Wang ^{a, b} ,
Shule Liu ^{c, *,} ,
Xiue Jiang ^{a, b, d, *,}

a.
State Key Laboratory of Electroanalytical Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, China
b.
School of Applied Chemistry and Engineering, University of Science and Technology of China, Hefei 230026, China
c.
School of Materials Science and Engineering, Sun Yat-sen University, Guangzhou 510275, China
d.
Research Center for Analytical Science, College of Chemistry, Nankai University, Tianjin 300071, China

liushle@mail.sysu.edu.cn

jiangxiue@ciac.ac.cn

Received Date: 6 January 2024
Revised Date: 4 April 2024
Accepted Date: 30 April 2024
Available Online: 1 May 2024

Figures(4)

Revealing the factors that affect the vibrational frequency of Stark probe at interface is a pre-requirement for evaluating the absolute interfacial electric field. Here using surface-enhanced infrared absorption (SEIRA) spectroscopy, attenuated total reflection (ATR) spectroscopy and molecular dynamics (MD), we reveal the assembled CN at gold nanofilm exhibits a reduced Stark tuning rate (STR) referring to the vibrational frequency shift in response to electric field comparing with the bulk which was regulated by the electron transfer between S and Au. These findings lead to a deeper understanding of the vibrational Stark effect at the interface and provide guidance for improving the interface electric field theory.
- Surface-enhanced infrared spectroscopy,
- Attenuated total reflection spectroscopy,
- Vibrational stark effect,
- Stark tuning rate,
- Cyano group
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