Citation: Jiawei Ge, Xian Wang, Heyuan Tian, Hao Wan, Wei Ma, Jiangying Qu, Junjie Ge. Iridium-based catalysts for oxygen evolution reaction in proton exchange membrane water electrolysis[J]. Chinese Chemical Letters, ;2025, 36(5): 109906. doi: 10.1016/j.cclet.2024.109906 shu

Iridium-based catalysts for oxygen evolution reaction in proton exchange membrane water electrolysis

Jiawei Ge ^{a, b} ,
Xian Wang ^b ,
Heyuan Tian ^b ,
Hao Wan ^b ,
Wei Ma ^c ,
Jiangying Qu ^{a, *,} ,
Junjie Ge ^{b, *,}

a.
Dongguan Key Laboratory of Low-Carbon Recycling and Utilization, School of Environment and Civil Engineering, Dongguan University of Technology, Dongguan 523808, China
b.
School of Chemistry and Materials Science, University of Science & Technology of China, Hefei 230026, China
c.
State Grid Anhui Electric Power Research Institute, Hefei 230601, China

qujianggaofeng@163.com

gejunjie@ustc.edu.cn

Received Date: 21 January 2024
Revised Date: 24 March 2024
Accepted Date: 17 April 2024
Available Online: 18 April 2024

Figures(10)

Proton exchange membrane water electrolysis (PEMWE) is a favorable technology for producing high-purity hydrogen under high current density using intermittent renewable energy. The performance of PEMWE is largely determined by the oxygen evolution reaction (OER), a sluggish four-electron reaction with a high reaction barrier. Nowadays, iridium (Ir)-based catalysts are the catalysts of choice for OER due to their excellent activity and durability in acidic solution. However, its high price and unsatisfactory electrochemical performance severely restrict the PEMWE’s practical application. In this review, we initiate by introducing the current OER reaction mechanisms, namely adsorbate evolution mechanism and lattice oxygen mechanism, with degradation mechanisms discussed. Optimized strategies in the preparation of advanced Ir-based catalysts are further introduced, with merits and potential problems also discussed. The parameters that determine the performance of PEMWE are then introduced, with unsolved issues and related outlooks summarized in the end.
- Iridium-based catalysts,
- Oxygen evolution reaction,
- Proton exchange membrane water electrolysis,
- Degradation mechanism,
- Optimized strategies,
- Practical application
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