Citation: Hao Zhang, Haonan Qu, Ehsan Bahojb Noruzi, Haibing Li, Feng Liang. A nanocomposite film with layer-by-layer self-assembled gold nanospheres driven by cucurbit[7]uril for the selective transport of L-tryptophan and lysozyme[J]. Chinese Chemical Letters, ;2025, 36(1): 109731. doi: 10.1016/j.cclet.2024.109731 shu

A nanocomposite film with layer-by-layer self-assembled gold nanospheres driven by cucurbit[7]uril for the selective transport of L-tryptophan and lysozyme

Hao Zhang ^{a, c} ,
Haonan Qu ^b ,
Ehsan Bahojb Noruzi ^b ,
Haibing Li ^{b, *,} ,
Feng Liang ^{a, *,}

a.
The State Key Laboratory of Refractories and Metallurgy, School of Chemistry and Chemical Engineering, Wuhan University of Science and Technology, Wuhan 430081, China
b.
National Key Laboratory of Green Pesticide, College of Chemistry, Central China Normal University, Wuhan 430079, China
c.
School of Environmental and Chemical Engineering, Jiangsu Ocean University, Lianyungang 222005, China

lhbing@mail.ccnu.edu.cn

feng_liang@whu.edu.cn

Received Date: 13 December 2023
Revised Date: 12 February 2024
Accepted Date: 22 February 2024
Available Online: 6 March 2024

Figures(5)

Selective separation of amino acids and proteins is crucial in various areas of research, including proteomics, protein structure and function studies, protein purification and drug development, and biosensing and biodetection. A nanocomposite film is formed by combining layer-by-layer self-assembled gold nanospheres (AuNPs) driven by cucurbit[7]uril (CB[7]) and polymethyl methacrylate (PMMA) film. Due to the host-guest interactions, the selective transmission of L-tryptophan in the nanocomposite film is confirmed by the current-voltage measurements using a picoammeter. Furthermore, by adjusting the particle size of AuNPs to increase channel size, lysozyme containing multiple tryptophan residues can selectively pass through the nanocomposite film, indicating the high versatility and adaptability of the nanocomposite film. This study will provide a new direction for the selective separation of amino acids and proteins.
- Nanocomposite film,
- Cucurbit[7]uril,
- Gold nanospheres,
- Host–guest interactions,
- Selective transmission
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