Citation: Hongliang Zeng, Yuan Ji, Jinfeng Wen, Xu Li, Tingting Zheng, Qiu Jiang, Chuan Xia. Pt nanocluster-catalyzed hydrogen evolution reaction: Recent advances and future outlook[J]. Chinese Chemical Letters, ;2025, 36(3): 109686. doi: 10.1016/j.cclet.2024.109686 shu

Pt nanocluster-catalyzed hydrogen evolution reaction: Recent advances and future outlook

Hongliang Zeng ^a ,
Yuan Ji ^a ,
Jinfeng Wen ^a ,
Xu Li ^a ,
Tingting Zheng ^a ,
Qiu Jiang ^{a, b, *,} ,
Chuan Xia ^{a, b, *,}

a.
School of Materials and Energy, University of Electronic Science and Technology of China, Chengdu 611731, China
b.
Yangtze Delta Region Institute (Huzhou), University of Electronic Science and Technology of China, Huzhou 313001, China

jiangqiu@uestc.edu.cn

chuan.xia@uestc.edu.cn

Received Date: 18 December 2023
Revised Date: 25 January 2024
Accepted Date: 29 February 2024
Available Online: 1 March 2024

Figures(16)

As hydrogen energy technologies gain momentum, the role of renewable energy in facilitating sustainable hydrogen production is becoming increasingly critical. As a hydrogen production method, water electrolysis has attracted much attention from researchers due to its operational simplicity, the high purity of the hydrogen generated, and its potential for achieving zero carbon emissions throughout the process. Numerous studies has been manipulated on platinum (Pt)-based catalysts, which exhibit superior performance in hydrogen evolution reactions. Within this category, Pt nanoclusters stand out due to their unique attributes, such as quantum size effects and unique coordination environments. These features enable them to outperform both Pt metal atoms and nanoparticles in hydrogen evolution reactions regarding activity and stability. Here, we primarily delve into the reaction mechanisms underlying Pt nanocluster-based hydrogen catalysts, with particular emphasis on the interactions between the metal catalysts and their associated support materials. We provide an exhaustive summary of the strategies employed in the synthesis, the structural analyses conducted, and the performance metrics observed for Pt nanocluster catalysts when paired with various supporting materials. In closing, we explore the future potential and challenges facing Pt nanocluster-based catalysts in the context of industrial water electrolysis, along with emerging avenues for their design and optimization.
- Platinum,
- Nanoclusters,
- Electronic interaction,
- Hydrogen evolution,
- Active sites
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沈阳化工大学材料科学与工程学院沈阳 110142