Citation: Qiyan Wu, Ruixin Zhou, Zhangyi Yao, Tanyuan Wang, Qing Li. Effective approaches for enhancing the stability of ruthenium-based electrocatalysts towards acidic oxygen evolution reaction[J]. Chinese Chemical Letters, ;2024, 35(10): 109416. doi: 10.1016/j.cclet.2023.109416 shu

Effective approaches for enhancing the stability of ruthenium-based electrocatalysts towards acidic oxygen evolution reaction

State Key Laboratory of Materials Processing and Die & Mould Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China

wangty@hust.edu.cn

qing_li@hust.edu.cn

Received Date: 7 November 2023
Revised Date: 29 November 2023
Accepted Date: 11 December 2023
Available Online: 20 December 2023

Figures(9)

Water splitting with proton exchange membrane water electrolyzers (PEMWE) is regarded as a promising pathway for sustainable hydrogen conversion. Additionally, oxygen evolution reaction (OER) is considered as the dominant factor during the whole process due to the sluggish kinetics. Among the catalysts, Ru-based catalysts draw special attention because of their excellent activity and relatively low price. However, the limited stability impedes their further commercialization and tremendous efforts have been devoted to overcome this challenge. This review firstly introduces the basic mechanisms of OER. Then the evaluation protocols and techniques to investigate the stability of Ru-based catalysts are summarized. A detailed elucidation of the possible degradation mechanisms is also critically analyzed. Furthermore, effective strategies to design durable Ru-based catalysts for acidic OER are discussed. Such as heteroatom doping, phase and facet engineering, heterostructure building and support optimization. Finally, promises, perspectives and challenges in developing highly durable Ru-based catalysts for acidic OER are outlined.
- Acidic oxygen evolution,
- Ru-based catalysts,
- Stability,
- Degradation mechanisms,
- Optimization strategies
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