Citation: Ningning Zhao, Yuyan Liang, Wenjie Huo, Xinyan Zhu, Zhangxing He, Zekun Zhang, Youtuo Zhang, Xianwen Wu, Lei Dai, Jing Zhu, Ling Wang, Qiaobao Zhang. Separator functionalization enables high-performance zinc anode via ion-migration regulation and interfacial engineering[J]. Chinese Chemical Letters, ;2024, 35(9): 109332. doi: 10.1016/j.cclet.2023.109332 shu

Separator functionalization enables high-performance zinc anode via ion-migration regulation and interfacial engineering

Ningning Zhao ^a ,
Yuyan Liang ^a ,
Wenjie Huo ^a ,
Xinyan Zhu ^a ,
Zhangxing He ^{a, *,} ,
Zekun Zhang ^a ,
Youtuo Zhang ^a ,
Xianwen Wu ^{b, *,} ,
Lei Dai ^a ,
Jing Zhu ^a ,
Ling Wang ^a ,
Qiaobao Zhang ^{c, *,}

a.
School of Chemical Engineering, North China University of Science and Technology, Tangshan 063009, China
b.
School of Chemistry and Chemical Engineering, Jishou University, Jishou 416000, China
c.
Department of Materials Science and Engineering, College of Materials, Xiamen University, Xiamen 361005, China

zxhe@ncst.edu.cn

wxwcsu2011@163.com

zhangqiaobao@xmu.edu.cn

Received Date: 26 October 2023
Revised Date: 10 November 2023
Accepted Date: 21 November 2023
Available Online: 22 November 2023

Figures(4)

Aqueous zinc ion batteries (AZIBs) are promising energy storage devices. However, the formation of dendrites, hydrogen evolution, and corrosion reaction seriously affect their electrochemical performance. Herein, the synergistic effect of ion-migration regulation and interfacial engineering has been confirmed as the potential strategy by kaolin functionalized glass fiber separator (KL-GF) to alleviate these problems. The rapid and orderly Zn²⁺ migration was achieved to improve the transfer kinetics and induced uniform zinc deposition by more zinc-philic sites of KL-GF. Based on the interfacial engineering, the side reactions were effectively mitigated and crystal planes were regulated through KL-GF. The hydrophilicity of KL alleviated the corrosion and hydrogen evolution. Importantly, a preferential orientation of Zn (002) crystal plane by KL-GF was induced to further realize dendrite-free deposition by density functional theory (DFT) and X-ray diffraction (XRD) characterization. Hence, the Zn|KL-GF|MnO₂ cell maintained a high discharge capacity of 96.8 mAh/g at 2 A/g after 1000 cycles. This work can provide guidance enabling high-performance zinc anode for AZIBs.
- Energy storage,
- Aqueous zinc ion batteries,
- Separators,
- Ion-migration regulation,
- Interfacial engineering
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