Citation: Zhenzhu Wang, Chenglong Liu, Yunpeng Ge, Wencan Li, Chenyang Zhang, Bing Yang, Shizhong Mao, Zeyuan Dong. Differentiated self-assembly through orthogonal noncovalent interactions towards the synthesis of two-dimensional woven supramolecular polymers[J]. Chinese Chemical Letters, ;2024, 35(5): 109127. doi: 10.1016/j.cclet.2023.109127 shu

Differentiated self-assembly through orthogonal noncovalent interactions towards the synthesis of two-dimensional woven supramolecular polymers

Zhenzhu Wang ^{a, b} ,
Chenglong Liu ^{a, b} ,
Yunpeng Ge ^{a, b} ,
Wencan Li ^{a, b} ,
Chenyang Zhang ^{a, b} ,
Bing Yang ^a ,
Shizhong Mao ^a ,
Zeyuan Dong ^{a, b, *,}

a.
State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry, Jilin University, Changchun 130012, China
b.
Center for Supramolecular Chemical Biology, Jilin University, Changchun 130012, China

zdong@jlu.edu.cn

Received Date: 5 June 2023
Revised Date: 12 September 2023
Accepted Date: 20 September 2023
Available Online: 21 September 2023

Figures(5)

Molecular weaving is a powerful approach to make molecularly woven materials that have showed unprecedented characteristics and properties intrinsically distinct to those of non-woven materials. We here report a facile and efficient approach for the synthesis of 2D woven supramolecular polymers by differentiated self-assembly through orthogonal noncovalent interactions. Importantly, the difference in binding strength of two orthogonal noncovalent interactions can be used to control the process of molecular weaving. Consequently, single-layered 2D woven supramolecular polymers were synthesized and fully characterized by various techniques. This study demonstrates a controllable method for molecular weaving, and will significantly hasten the development of molecularly woven materials.
- Differentiated self-assembly,
- Double-stranded helix,
- Molecular weaving,
- Supramolecular chemistry,
- Two-dimensional polymer
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