Citation: Xianxu Chu, Lu Wang, Junru Li, Hui Xu. Surface chemical microenvironment engineering of catalysts by organic molecules for boosting electrocatalytic reaction[J]. Chinese Chemical Letters, ;2024, 35(8): 109105. doi: 10.1016/j.cclet.2023.109105 shu

Surface chemical microenvironment engineering of catalysts by organic molecules for boosting electrocatalytic reaction

Xianxu Chu ^{a, *,} ,
Lu Wang ^a ,
Junru Li ^a ,
Hui Xu ^b

a.
Henan Key Laboratory of Biomolecular Recognition and Sensing, College of Chemistry and Chemical Engineering, Shangqiu Normal University, Shangqiu 476000, China
b.
Key Laboratory of Advanced Catalytic Materials and Technology, Advanced Catalysis and Green Manufacturing Collaborative Innovation Center, Changzhou University, Changzhou 213164, China

xxchu13633@163.com

Received Date: 29 March 2023
Revised Date: 15 August 2023
Accepted Date: 14 September 2023
Available Online: 16 September 2023

Figures(11)

Electrocatalysis is a surface-sensitive process, in which the catalytic activity of electrocatalyst highly relates to the surface adsorption/desorption behaviors of the reactants/intermediates/products on the catalytically active sites. Surface chemical microenvironment engineering via organic molecules functionalization is a promising strategy to tune the electrocatalytic activity since it can well modify the electrode/electrolyte interface and alter the reaction pathways. In this review, we summarize the recent progress of surface microenvironment engineering of electrocatalysts induced by organic molecules functionalization, with the special focus on the organic molecule-assisted growth mechanism and unique electronic effect. More importantly, the applications of organic molecule functionalized catalysts in various electrocatalytic reactions are also systematically summarized, along with a deep discussion on the conclusion and perspective. This work will open a new avenue for the construction and modification of advanced electrocatalysts based on organic molecule-mediated interface engineering.
- Chemical microenvironment engineering,
- Organic molecules,
- Electrocatalysis,
- Functionalization Interface
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沈阳化工大学材料科学与工程学院沈阳 110142