Citation: Yan-Hu Wang, Ke-Wei Tong, Chao-Qin Chen, Jing Du, Peng Yang. Weak interaction-steered evolution of polyoxovanadate-based metal-organic polyhedra from transformation via interlock to packing[J]. Chinese Chemical Letters, ;2024, 35(2): 109066. doi: 10.1016/j.cclet.2023.109066 shu

Weak interaction-steered evolution of polyoxovanadate-based metal-organic polyhedra from transformation via interlock to packing

Yan-Hu Wang ^{a, 1} ,
Ke-Wei Tong ^{a, 1} ,
Chao-Qin Chen ^a ,
Jing Du ^{b, *,} ,
Peng Yang ^{a, *,}

a.
College of Chemistry and Chemical Engineering, Advanced Catalytic Engineering Research Center of the Ministry of Education, Hunan University, Changsha 410082, China
b.
College of Chemistry and Materials Science, Testing and Analysis Center, Hebei Normal University, Shijiazhuang 050024, China

duj622@hebtu.edu.cn

pengyang216@hnu.edu.cn

Received Date: 25 July 2023
Revised Date: 14 August 2023
Accepted Date: 7 September 2023
Available Online: 9 September 2023

Figures(5)

A bottleneck in biomimetic synthesis consists in the full copy of, for example, the hierarchical structure of proteins directed by weak interactions. By contrast with covalent bonds bearing definite orientation and high stability, weak intermolecular forces within a continuous dynamic equilibrium can be hardly tamed for molecular design. In this endeavor, a ligand-dominated strategy that embodies tunable electrostatic repulsion and π…π stacking was first employed to shape polyoxovanadate-based metal-organic polyhedra (VMOPs). Structural evolution involving transformation, interlock, and discovery of an unprecedented prototype of the Star of David was hence achievable. Not only as a handy tool for the primary structural control over VMOPs, these weak forces allow for an advanced management on the spatial distribution of such manmade macromolecules as well as the associated physicochemical behaviors, representing an ideal model for simulating and interpreting the conformation-function relationship of proteins.
- Polyoxometalates,
- Polyoxovanadates,
- Metal-organic polyhedron,
- Interlock,
- Weak intermolecular forces
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