Citation: Shuo Li, Xinran Liu, Yongjie Zheng, Jun Ma, Shijie You, Heshan Zheng. Effective peroxydisulfate activation by CQDs-MnFe₂O₄@ZIF-8 catalyst for complementary degradation of bisphenol A by free radicals and non-radical pathways[J]. Chinese Chemical Letters, ;2024, 35(5): 108971. doi: 10.1016/j.cclet.2023.108971 shu

Effective peroxydisulfate activation by CQDs-MnFe₂O₄@ZIF-8 catalyst for complementary degradation of bisphenol A by free radicals and non-radical pathways

Shuo Li ^a ,
Xinran Liu ^a ,
Yongjie Zheng ^a ,
Jun Ma ^b ,
Shijie You ^{b, *,} ,
Heshan Zheng ^{a, *,}

a.
College of Chemistry and Chemical Engineering, Qiqihar University, Qiqihar 161006, China
b.
State Key Laboratory of Urban Water Resource and Environment, School of Environment, Harbin Institute of Technology, Harbin 150090, China

sjyou@hit.edu.cn

787672849@qq.com

Received Date: 27 March 2023
Revised Date: 14 August 2023
Accepted Date: 24 August 2023
Available Online: 25 August 2023

Figures(6)

The present study reported fabrication of novel carbon quantum dots-MnFe₂O₄@ZIF-8 (CQDs-MFO@ZIF-8) by using co-precipitation hydrothermal method for activation of peroxydisulfate (PDS) to degrade bisphenol A (BPA), one of important emerging organic pollutants in water environment. CQDs-MFO@ZIF-8 served as a highly efficient thermal activated PDS catalyst with high catalytic degradation efficiency, reusability and stability. The catalyst achieved almost completely removal of 20.0 mg/L BPA within 5.0 min, and the degradation efficiency remained higher than 83% after 5 consecutive cycles. Free radicals (^•OH, SO₄^•− and ^•O₂⁻) and non-free radicals (¹O₂) were generated in the thermal PDS-activation system, in which singlet oxygen (¹O₂) played a dominant role in the degradation of BPA. The potential toxicity of BPA degradation intermediates was analyzed upon the culture of E. coli and Chlorella sorokiniana by using Ecological Structure-Activity Relationship Model (ECOSAR) program. The catalytic performances of BPA degradation by CQDs-MFO@ZIF-8 were evaluated for treatment of different practical water samples to further verify the feasibility of practical applications. This study provides proof-in-concept demonstration of new nanomaterials for enhanced catalytic water decontamination.
- Bisphenol A,
- Degradation,
- Peroxydisulfate,
- ¹O₂,
- Toxicity analysis
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沈阳化工大学材料科学与工程学院沈阳 110142

Effective peroxydisulfate activation by CQDs-MnFe2O4@ZIF-8 catalyst for complementary degradation of bisphenol A by free radicals and non-radical pathways

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通讯作者: 陈斌, bchen63@163.com

Effective peroxydisulfate activation by CQDs-MnFe₂O₄@ZIF-8 catalyst for complementary degradation of bisphenol A by free radicals and non-radical pathways