Citation: Yue Qian, Zhoujia Liu, Haixin Song, Ruize Yin, Hanni Yang, Siyang Li, Weiwei Xiong, Saisai Yuan, Junhao Zhang, Huan Pang. Imide-based covalent organic framework with excellent cyclability as an anode material for lithium-ion battery[J]. Chinese Chemical Letters, ;2024, 35(6): 108785. doi: 10.1016/j.cclet.2023.108785 shu

Imide-based covalent organic framework with excellent cyclability as an anode material for lithium-ion battery

Yue Qian ^{a, 1} ,
Zhoujia Liu ^{a, 1} ,
Haixin Song ^a ,
Ruize Yin ^a ,
Hanni Yang ^a ,
Siyang Li ^a ,
Weiwei Xiong ^{a, c, *,} ,
Saisai Yuan ^{a, *,} ,
Junhao Zhang ^a ,
Huan Pang ^{b, *,}

a.
School of Environmental & Chemical Engineering, Jiangsu University of Science and Technology, Zhenjiang 212003, China
b.
School of Chemistry & Chemical Engineering, Yangzhou University, Yangzhou 225009, China
c.
Shandong Key Laboratory of Biochemical Analysis, College of Chemistry and Molecular Engineering, Qingdao University of Science and Technology, Qingdao 266042, China

xiongweiwei@just.edu.cn

yuansaisai@just.edu.cn

huanpangchem@hotmail.com

Received Date: 22 April 2023
Revised Date: 14 June 2023
Accepted Date: 5 July 2023
Available Online: 6 July 2023

Figures(4)

Covalent organic frameworks (COFs) exhibiting reversible redox behaviors have been identified as promising candidates for constructing electrode materials in lithium-ion batteries (LIBs). However, their extensive application has been limited due to finite redox sites and poor structural stability. In this study, we design and synthesize a novel polyimide covalent organic framework (PI-COF) using the traditional solvothermal method and successfully apply it as an anode material for LIBs. The large conjugated structure of PI-COF accelerates charge transfer, while its large surface area provides more active sites, making PI-COF an attractive anode material for LIBs. Furthermore, the PI-COF anode material demonstrates high reversible specific capacity and excellent long-term cycling stability due to its COF characteristics. Specifically, the PI-COF electrodes deliver a specific capacity of 800 mAh/g at a current density of 200 mA/g after 200 cycles, while a specific capacity of 450 mAh/g at a current density of 1000 mA/g is sustained after 800 cycles. The outstanding lithium storage capacity, particularly the satisfactory long-term cycling stability, establishes PI-COF as a promising material for LIBs.
- Ethylenediaminetetraacetic dianhydride,
- Covalent organic frameworks,
- Polyimide,
- Lithium-ion battery,
- Anode material
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