Citation: Dong Cheng, Youyou Feng, Bingxi Feng, Ke Wang, Guoxin Song, Gen Wang, Xiaoli Cheng, Yonghui Deng, Jing Wei. Polyphenol-mediated interfacial deposition strategy for supported manganese oxide catalysts with excellent pollutant degradation performance[J]. Chinese Chemical Letters, ;2024, 35(5): 108623. doi: 10.1016/j.cclet.2023.108623 shu

Polyphenol-mediated interfacial deposition strategy for supported manganese oxide catalysts with excellent pollutant degradation performance

Dong Cheng ^a ,
Youyou Feng ^a ,
Bingxi Feng ^a ,
Ke Wang ^b ,
Guoxin Song ^c ,
Gen Wang ^{b, *,} ,
Xiaoli Cheng ^d ,
Yonghui Deng ^c ,
Jing Wei ^{a, *,}

a.
The Key Laboratory of Biomedical Information Engineering of Ministry of Education, State Key Lab of Transducer Technology, School of Life Science and Technology, Xi'an Jiaotong University, Xi'an 710049, China
b.
School of Environmental and Municipal Engineering, Xi'an University of Architecture and Technology, Xi'an 710055, China
c.
Department of Chemistry, State Key Laboratory of Molecular Engineering of Polymers, State Key Laboratory of Transducer Technology, Fudan University, Shanghai 200433, China
d.
Key Laboratory of Functional Inorganic Material Chemistry, Ministry of Education, School of Chemistry and Materials Science, Heilongjiang University, Harbin 150080, China

wanggen@xauat.edu.cn

jingwei@xjtu.edu.cn

Received Date: 25 March 2023
Revised Date: 22 May 2023
Accepted Date: 29 May 2023
Available Online: 3 June 2023

Figures(4)

In persulfate-based advanced oxidation process (PS-AOPs), fixing nanosized metal oxide on processable substrates is highly desirable to avoid the aggregation and loss of nanocatalysts during the practical application. However, it is still challenging to develop a versatile strategy for the deposition of metal oxide nanocatalysts on various substrates with different physicochemical properties. Herein, polyphenols are utilized as a "molecular glue" and reductant to mediate the interfacial deposition of MnO₂ nanocatalysts on different substrates. MnO₂ nanocatalysts were in-situ grown on macroscope mineral substrates (e.g., airstone) via an interfacial redox strategy between tannic acid (TA) and oxidized KMnO₄, and then employed as a fixed catalyst of peroxymonosulfate (PMS) activation for treating pharmaceutical and personal care products (PPCPs) in water. The fixed MnO₂ exhibited superior catalytic performance toward different PPCPS via a singlet oxygen (¹O₂)-dominated nonradical oxidation pathway. PPCPs in the secondary effluent of wastewater treatment plants could be effectively removed by a fixed-bed column of the fixed MnO₂ with long term stability. Redox cycle of Mn⁴⁺/Mn³⁺ and surface hydroxyl group of the fixed MnO₂ was proved to be responsible for the activation of PMS. This work provides a new avenue for developing fixed metal oxides for sustainable water treatment.
- Redox strategy,
- Manganese oxides,
- Fixed catalyst,
- Peroxymonosulfate,
- PPCPs
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