Citation: Xiping Dong, Xuan Wang, Zhixiu Lu, Qinhao Shi, Zhengyi Yang, Xuan Yu, Wuliang Feng, Xingli Zou, Yang Liu, Yufeng Zhao. Construction of Cu-Zn Co-doped layered materials for sodium-ion batteries with high cycle stability[J]. Chinese Chemical Letters, ;2024, 35(5): 108605. doi: 10.1016/j.cclet.2023.108605 shu

Construction of Cu-Zn Co-doped layered materials for sodium-ion batteries with high cycle stability

Xiping Dong ^{a, 1} ,
Xuan Wang ^{b, 1} ,
Zhixiu Lu ^a ,
Qinhao Shi ^a ,
Zhengyi Yang ^a ,
Xuan Yu ^a ,
Wuliang Feng ^a ,
Xingli Zou ^c ,
Yang Liu ^{a, *,} ,
Yufeng Zhao ^{a, *,}

a.
Institute for Sustainable Energy & College of Sciences, Shanghai University, Shanghai 200444, China
b.
Key Laboratory for Advanced Technology in Environmental Protection of Jiangsu Province, Yancheng Institute of Technology, Yancheng 224051, China
c.
State Key Laboratory of Advanced Special Steel & Shanghai Key Laboratory of Advanced Ferrometallurgy & School of Materials Science and Engineering, Shanghai University, Shanghai 200444, China

Yangliu45@shu.edu.cn

yufengzhao@shu.edu.cn

Received Date: 23 April 2023
Revised Date: 16 May 2023
Accepted Date: 23 May 2023
Available Online: 25 May 2023

Figures(6)

Due to its high operational voltage and energy density, P2-type Na_0.67Ni_0.3Mn_0.7O₂ has become a leading cathode material for sodium-ion batteries (SIBs), which is an ideal option for large-scale energy storage. However, the practical application of P2-type Na_0.67Ni_0.3Mn_0.7O₂ is limited by the capacity constraints and unwanted phase transitions, presenting significant challenges to the widespread application of SIBs. To address these challenges and optimize the electrochemical properties of the P2 phase cathode material, this study proposes a Cu and Zn co-doped strategy to improve the electrochemical performance. The incorporation of Cu/Zn can stabilize the P2-phase structure against P2-O2 phase transitions, thus enhancing its electrochemical properties. The as-obtained P2-type Na_0.67[Ni_0.3Mn_0.58Cu_0.09Zn_0.03]O₂ cathode material shows an impressive cycling stability, maintaining 80% capacity retention after 1000 cycles at 2 C. The cyclic voltammetry (CV) tests show that the Cu²⁺/Cu³⁺ redox reaction is also involved in charge compensation during the charge/discharge process.
- Sodium-ion batteries,
- Cathode material,
- Cycle performance,
- Cu/Zn co-doped,
- P2-type Na_0.67Ni_0.3Mn_0.7O₂
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