Citation: Botao Gao, He Qi, Hui Liu, Jun Chen. Role of polarization evolution in the hysteresis effect of Pb-based antiferroelecrtics[J]. Chinese Chemical Letters, ;2024, 35(4): 108598. doi: 10.1016/j.cclet.2023.108598 shu

Role of polarization evolution in the hysteresis effect of Pb-based antiferroelecrtics

Botao Gao ^{a, b} ,
He Qi ^a ,
Hui Liu ^{a, *,} ,
Jun Chen ^{a, c, *,}

a.
Beijing Advanced Innovation Center for Materials Genome Engineering, Department of Physical Chemistry, University of Science and Technology Beijing, Beijing 100083, China
b.
Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 201899, China
c.
Hainan University, Haikou 570228, China

huiliu@ustb.edu.cn

junchen@ustb.edu.cn

Received Date: 25 March 2023
Revised Date: 25 April 2023
Accepted Date: 22 May 2023
Available Online: 23 May 2023

Figures(4)

The electric field-induced irreversible domain wall motion results in a ferroelectric (FE) hysteresis. In antiferroelectrics (AFEs), the irreversible phase transition is the main reason for the hysteresis effects, which plays an important role in energy storage performance. Compared to the well-demonstrated FE hysteresis, the structural mechanism of the hysteresis in AFE is not well understood. In this work, the underlying correlation between structure and the hysteresis effect is unveiled in Pb(Zr, Sn, Ti)O₃ AFE system by using in-situ electrical biasing synchrotron X-ray diffraction. It is found that the AFE with a canting dipole configuration, which shows a continuous polarization rotation under the electric field, tends to have a small hysteresis effect. It presents a negligible phase transition, a small axis ratio, and electric field-induced lattice changing, small domain switching. All these features together lead to a slim hysteresis loop and a high energy storage efficiency. These results offer a deep insight into the structure-hysteresis relationship of AFEs and are helpful for the design of energy storage material.
- Antiferroelectric,
- Hysteresis effect,
- Structure refinement,
- Perovskite,
- In situ synchrotron radiation
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