Citation: Fanjun Kong, Yixin Ge, Shi Tao, Zhengqiu Yuan, Chen Lu, Zhida Han, Lianghao Yu, Bin Qian. Engineering and understanding SnS_0.5Se_0.5@N/S/Se triple-doped carbon nanofibers for enhanced sodium-ion batteries[J]. Chinese Chemical Letters, ;2024, 35(4): 108552. doi: 10.1016/j.cclet.2023.108552 shu

Engineering and understanding SnS_0.5Se_0.5@N/S/Se triple-doped carbon nanofibers for enhanced sodium-ion batteries

Fanjun Kong ^{a, c} ,
Yixin Ge ^a ,
Shi Tao ^{a, *,} ,
Zhengqiu Yuan ^c ,
Chen Lu ^a ,
Zhida Han ^a ,
Lianghao Yu ^{b, *,} ,
Bin Qian ^{a, *,}

a.
School of Electronic and Information Engineering, Changshu Institute of Technology, Changshu 215500, China
b.
Key Laboratory of Spin Electron and Nanomaterials of Anhui Higher Education Institutes, Suzhou University, Suzhou 234000, China
c.
Far East Holding Group Co., Ltd., Yixing 214200, China

taoshi@cslg.edu.cn

lhyu@ahszu.edu.cn

njqb@cslg.edu.cn

Received Date: 27 February 2023
Revised Date: 30 March 2023
Accepted Date: 8 May 2023
Available Online: 11 May 2023

Figures(4)

Tin-based chalcogenides have attracted tremendous attention as an anode material for sodium storage owing to their unique structure and high theoretical capacity. Unfortunately, the large volume change and poor conductivity lead to sluggish reaction kinetics and poor cycling performance. Herein, SnS_0.5Se_0.5 nanoparticles coupled with N/S/Se triple-doped carbon nanofibers (SnS_0.5Se_0.5@NSSe-C) are designed and synthesized through electrospinning and annealing process. Benefiting from the synergistic effects of SnS_0.5Se_0.5 and NSSe-C, the SnS_0.5Se_0.5@NSSe-C nanofibers exhibit a high reversible capacity and ultralong cycle life at higher current density for sodium-ion batteries. Furthermore, the sodium storage mechanism and electrochemical reaction kinetics of the SnS_0.5Se_0.5@NSSe-C composite are characterized by the in-situ measurements. The theoretical calculations further reveal the structural advantages of SnS_0.5Se_0.5@NSSe-C composite, which exhibits a high adsorption energy of Na⁺. This work can provide a novel idea for the synthesis of ternary tin-based chalcogenides and is beneficial for the investigation of their reaction kinetics.
- SnS_0.5Se_0.5,
- Carbon nanofibers,
- Doping,
- Density functional theory,
- Sodium ion batteries
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通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142

Engineering and understanding SnS0.5Se0.5@N/S/Se triple-doped carbon nanofibers for enhanced sodium-ion batteries

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通讯作者: 陈斌, bchen63@163.com

Engineering and understanding SnS_0.5Se_0.5@N/S/Se triple-doped carbon nanofibers for enhanced sodium-ion batteries