Citation: Yanan Chen, Jiao Lei, Yanling Zhai, Zhijun Zhu, Weitai Wu, Xiaoquan Lu. Tungsten oxide nanowires and polyaniline hybrid film-based electrochromic device with multicolor display and enhanced capacitance[J]. Chinese Chemical Letters, ;2023, 34(11): 108305. doi: 10.1016/j.cclet.2023.108305 shu

Tungsten oxide nanowires and polyaniline hybrid film-based electrochromic device with multicolor display and enhanced capacitance

Yanan Chen ^{a, 1} ,
Jiao Lei ^{a, 1} ,
Yanling Zhai ^{a, *,} ,
Zhijun Zhu ^{b, *,} ,
Weitai Wu ^c ,
Xiaoquan Lu ^{a, *,}

a.
Institute of Molecular Metrology, College of Chemistry and Chemical Engineering, Qingdao University, Qingdao 266071, China
b.
Institute of Hybrid Materials, National Center of International Research for Hybrid Materials Technology, National Base of International Science & Technology Cooperation, College of Materials Science and Engineering, Qingdao University, Qingdao 266071, China
c.
State Key Laboratory of Physical Chemistry of Solid Surfaces, Xiamen University, Xiamen 361005, China

zhaiyanling@qdu.edu.cn

zhuzhijun@qdu.edu.cn

luxq@nwnu.edu.cn

Received Date: 25 October 2022
Revised Date: 6 February 2023
Accepted Date: 5 March 2023
Available Online: 12 March 2023

Figures(4)

Electrochromic devices (ECDs) have exhibited promising applications in the fields of energy-saving intelligent buildings and next-generation displays because of their simple structure, low power consumption, and multicolor displays. W₁₈O₄₉/polyaniline (PANI) hybrid films are prepared and assembled to ECDs. Compared with pure PANI and W₁₈O₄₉ films, the hybrid film exhibits superior electrochemical and electrochromic performance, including high optical modulation (70.2%), large areal capacity (79.6 mF/cm²), and good capacitance retention. The excellent electrochemical and electrochromic performance is ascribed to the formation of the donor (PANI)-acceptor (W₁₈O₄₉) pair, the porous structure in the nanowires, and the large surface area, which enhance electron delocalization of the W₁₈O₄₉/PANI, improve the ion diffusion rate, and increase the charge storage sites. Furthermore, benefitting from the outstanding optical, electrical, and multifunctional properties, the W₁₈O₄₉/PANI hybrid film-based ECD platform is expected to play an important role in electrochromism and energy storage.
- W₁₈O₄₉/PANI,
- Electrochromism,
- Multifunctional devices,
- Multicolor,
- Energy storage
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