Citation: Yujiao Kan, Ruxin Zhang, Xing Xu, Bo Wei, Yanan Shang. Comparative study of raw and HNO₃-modified porous carbon from waste printed circuit boards for sulfadiazine adsorption: Experiment and DFT study[J]. Chinese Chemical Letters, ;2023, 34(7): 108272. doi: 10.1016/j.cclet.2023.108272 shu

Comparative study of raw and HNO₃-modified porous carbon from waste printed circuit boards for sulfadiazine adsorption: Experiment and DFT study

Yujiao Kan ^a ,
Ruxin Zhang ^{a, b} ,
Xing Xu ^c ,
Bo Wei ^{a, d} ,
Yanan Shang ^{a, *,}

a.
School of Safety and Environmental Engineering, Shandong University of Science and Technology, Qingdao 266590, China
b.
Faculty of Light Industry, Qilu University of Technology (Shandong Academy of Sciences), Ji'nan 250353, China
c.
Shandong Key Laboratory of Water Pollution Control and Resource Reuse, School of Environmental Science and Engineering, Shandong University, Qingdao 266237, China
d.
Environment Research Institute, Shandong University, Qingdao 266237, China

shangyanan@sdust.edu.cn

Received Date: 13 December 2022
Revised Date: 22 February 2023
Accepted Date: 24 February 2023
Available Online: 26 February 2023

Figures(4)

A huge amount of waste printed circuit boards (WPCBs) was produced while the electronic manufacturing industry developed rapidly. WPCBs mainly consist of organic compounds, which makes it possible to prepare them into porous carbon as valuable adsorbent. However, WPCBs are also rich in valuable metals. Cu makes up the most of these metals. It is worth studying whether the residual metal will affect the application of carbon materials. In this study, the porous active carbon (AC) was prepared from WPCBs as an adsorbent. Sulfadiazine (SD), a widely detected antibiotic contaminant, was used as a target pollutant. Nitric acid (HNO₃) was used to modify AC (AC-HNO₃) to remove the residual Cu. The experiment results showed that the adsorption kinetics of SD by AC (k = 0.0025) and AC-HNO₃ (k = 0.0029) can be described better using a pseudo-second-order kinetic equation. The adsorption isotherms of AC and AC-HNO₃ on SD could be fitted by the Langmuir model. AC had a larger adsorption capacity than AC-HNO₃. Density functional theory (DFT) calculation results suggested that the −OH group and Cu on the surface of AC could be the adsorption sites and promote the SD adsorption. This work provides practical methods to recycle WPCBs into wealth and realized waste control by waste.
- WPCBs,
- DFT,
- Sulfadiazine,
- Porous carbon
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Comparative study of raw and HNO3-modified porous carbon from waste printed circuit boards for sulfadiazine adsorption: Experiment and DFT study

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通讯作者: 陈斌, bchen63@163.com

Comparative study of raw and HNO₃-modified porous carbon from waste printed circuit boards for sulfadiazine adsorption: Experiment and DFT study