Citation: Xinjiang Hu, Daixi Zhou, Hui Wang, Wenlong Zhang, Haoxiang Zhong, Yongsheng Chen. Preparation and characterization of M₁-N_x-C_y based single atom catalysts for environmental applications[J]. Chinese Chemical Letters, ;2023, 34(8): 108050. doi: 10.1016/j.cclet.2022.108050 shu

Preparation and characterization of M₁-N_x-C_y based single atom catalysts for environmental applications

Xinjiang Hu ^{a, b, *,} ,
Daixi Zhou ^a ,
Hui Wang ^a ,
Wenlong Zhang ^{b, c} ,
Haoxiang Zhong ^a ,
Yongsheng Chen ^{b, **,}

a.
College of Environmental Science and Engineering, Central South University of Forestry and Technology, Changsha 410004, China
b.
School of Civil and Environmental Engineering, Georgia Institute of Technology, Atlanta, GA 30332, United States
c.
Georgia Tech Shenzhen Institute, Tianjin University, Shenzhen 518067, China

^**

xjhu@csuft.edu.cn

yongsheng.chen@ce.gatech.edu

Received Date: 31 August 2022
Revised Date: 18 November 2022
Accepted Date: 6 December 2022
Available Online: 8 December 2022

Figures(8)

Single atom catalysts (SACs) have become the frontier research fields in catalysis. The M₁-N_x-C_y based SACs, wherein single metal atoms (M₁) are stabilized by N-doped carbonaceous materials, have provided new opportunities for catalysis due to their high reactivity, maximized atomic utilization, and high selectivity. In this review, the fabrication methods of M₁-N_x-C_y based SACs via support anchoring strategy and coordination design strategy are summarized to help the readers understand the interaction mechanism of single atoms and support. Then, characterization technologies for identifying single metal atoms are presented. Besides, the environmental applications including management of harmful gases, water purification are discussed. Finally, future opportunities and challenges for preparation strategies, mechanisms and applications are concluded. We conclude this review by emphasizing the fact that M₁-N_x-C_y based SACs has the potential to become an important candidate for solving current and future environmental pollution problems.
- Single atom catalysts,
- Photocatalysis,
- Electrocatalysis,
- Environmental applications
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Preparation and characterization of M1-Nx-Cy based single atom catalysts for environmental applications

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通讯作者: 陈斌, bchen63@163.com

Preparation and characterization of M₁-N_x-C_y based single atom catalysts for environmental applications