Citation: Chao Tan, Rui Tao, Zhihao Yang, Lei Yang, Xiaolei Huang, Yong Yang, Fei Qi, Zegao Wang. Tune the photoresponse of monolayer MoS₂ by decorating CsPbBr₃ perovskite nanoparticles[J]. Chinese Chemical Letters, ;2023, 34(7): 107979. doi: 10.1016/j.cclet.2022.107979 shu

Tune the photoresponse of monolayer MoS₂ by decorating CsPbBr₃ perovskite nanoparticles

Chao Tan ^a ,
Rui Tao ^a ,
Zhihao Yang ^a ,
Lei Yang ^a ,
Xiaolei Huang ^b ,
Yong Yang ^b ,
Fei Qi ^c ,
Zegao Wang ^{a, *,}

a.
College of Materials Science and Engineering, Sichuan University, Chengdu 610065, China
b.
State Key Laboratory of Solidification Processing, Center of Advanced Lubrication and Seal Materials, Northwestern Polytechnical University, Xi'an 710072, China
c.
College of Optoelectronic Engineering, Chongqing University of Posts and Telecommunications, Chongqing 400065, China

zegao@scu.edu.cn

Received Date: 17 September 2022
Revised Date: 29 October 2022
Accepted Date: 2 November 2022
Available Online: 5 November 2022

Figures(5)

Tuning the photoresponse of monolayer MoS₂ could extend its potential application in many fields, however, it is still a challenge. In this study, CsPbBr₃ nanoparticles were prepared and spin-coated on the surface of monolayer MoS₂ to fabricate hybrid CsPbBr₃/MoS₂ photodetectors. By combing the photoelectrical property of the CsPbBr₃, the synergistic effect has been systematically studied from its carrier mobility, photoresponse and detectivity. It was found that nanofilm-coating of CsPbBr₃ would impede the photoelectric performance due to the electron-hole recombination facilitated by the defects at the interface of CsPbBr₃ and MoS₂ films. While the nanoparticles decorating was observed to significantly improve the conductivity of the monolayer MoS₂, which also increased the on/off ratio of the MoS₂ transistor from 8.2 × 10³ to 4.4 × 10⁴, and enhanced the carrier mobility from 0.090 cm² V⁻¹ s⁻¹ to 0.202 cm² V⁻¹ s⁻¹, ascribing to a mixed electron recombination-injection process. Furthermore, the CsPbBr₃ nanofilm would decrease the responsivity to 136 and 178 A/W under the light wavelength of 400 and 500 nm, respectively, while decorating CsPbBr₃ nanoparticles improve the photoresponse to 948 and 883 A/W with the detectivity at the level of 10¹¹ Jones. This work may provide an easy and cost-efficient way to tune the photoresponse of MoS₂ photodetectors.
- MoS₂ photodetector,
- CsPbBr₃ NPs,
- Surface charge doping,
- Carrier mobility,
- Photoresponse
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Tune the photoresponse of monolayer MoS₂ by decorating CsPbBr₃ perovskite nanoparticles