Citation: Gaopeng Liu, Lin Wang, Bin Wang, Xingwang Zhu, Jinman Yang, Pengjun Liu, Wenshuai Zhu, Ziran Chen, Jiexiang Xia. Synchronous activation of Ag nanoparticles and BiOBr for boosting solar-driven CO₂ reduction[J]. Chinese Chemical Letters, ;2023, 34(6): 107962. doi: 10.1016/j.cclet.2022.107962 shu

Synchronous activation of Ag nanoparticles and BiOBr for boosting solar-driven CO₂ reduction

Gaopeng Liu ^{b, 1} ,
Lin Wang ^{b, 1} ,
Bin Wang ^b ,
Xingwang Zhu ^b ,
Jinman Yang ^b ,
Pengjun Liu ^{a, *,} ,
Wenshuai Zhu ^{b, *,} ,
Ziran Chen ^c ,
Jiexiang Xia ^{b, *,}

a.
Key Laboratory of Medicinal and Edible Plants Resources of Hainan Province, Hainan vocational university of Science and Technology, Haikou 571126, China
b.
School of Chemistry and Chemical Engineering, Institute for Energy Research, Jiangsu University, Zhenjiang 212013, China
c.
Department of Architecture and Environment Engineering, Sichuan Vocational and Technical College, Suining 629000, China

liupj12@126.com

zhuws@ujs.edu.cn

xjx@ujs.edu.cn

Received Date: 13 June 2022
Revised Date: 13 October 2022
Accepted Date: 27 October 2022
Available Online: 31 October 2022

Figures(4)

Artificial photosynthesis of valuable chemicals from CO₂ is a potential way to achieve sustainable carbon cycle. The CO₂ conversion activity is still inhibited by the sluggish charge kinetics and poor CO₂ activation. Herein, Ag nanoparticles coupled BiOBr have been constructed by in-situ photoreduction strategy. The crafting of interface between Ag nanoparticles and BiOBr nanosheets, achieving an ultra-fast charge transfer. The BiOBr semiconductor excited electrons and plasmonic Ag nanoparticles generated high-energy hot electrons synchronous accelerates the C=O double bond activation. Thus, the optimized Ag/BiOBr-2 heterostructure shows excellent CO₂ photoreduction activity with CO production of 133.75 and 6.83 µmol/g under 5 h of 300 W Xe lamp and visible light (λ > 400 nm) irradiation, which is 1.51 and 2.81 folds versus the pristine BiOBr, respectively. The mechanism of CO₂ photoreduction was in-depth understood through in-situ FT-IR spectrum and density functional theory calculations. This study provides some new perspectives into efficient photocatalytic CO₂ reduction.
- Ag nanoparticles,
- BiOBr,
- Hot electrons,
- Charge transfer,
- CO₂ photoreduction
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沈阳化工大学材料科学与工程学院沈阳 110142

Synchronous activation of Ag nanoparticles and BiOBr for boosting solar-driven CO2 reduction

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通讯作者: 陈斌, bchen63@163.com

Synchronous activation of Ag nanoparticles and BiOBr for boosting solar-driven CO₂ reduction