Citation: Hanyu Hu, Jiangbo Xi. Single-atom catalysis for organic reactions[J]. Chinese Chemical Letters, ;2023, 34(6): 107959. doi: 10.1016/j.cclet.2022.107959 shu

Single-atom catalysis for organic reactions

Hanyu Hu ,
Jiangbo Xi ^*,

Key Laboratory of Novel Biomass-Based Environmental and Energy Materials in Petroleum and Chemical Industry, Key Laboratory of Green Chemical Engineering Process of Ministry of Education, Engineering Research Center of Phosphorus Resources Development and Utilization of Ministry of Education, Hubei Key Laboratory of Novel Reactor and Green Chemical Technology, School of Chemistry and Environmental Engineering, Wuhan Institute of Technology, Wuhan 430205, China

Author Bio: Hanyu Hu is currently pursuing his master degree under the supervision of Prof. Jiangbo Xi at Wuhan Institute of Technology (WIT). He received B.S. degree in applied chemistry from WIT, China, in 2020. His research interests mainly include the design and synthesis of single-atom catalysts as well as metal-free carbocatalysts for organic reactions
Jiangbo Xi is currently a distinguished professor in the School of Chemistry and Environmental Engineering at Wuhan Institute of Technology (WIT), China. He obtained his B.S. and M.S. degrees from WIT, and his Ph.D. degree in 2015 from University of Huazhong University of Science and Technology, China. His current research topics are focused on the design and synthesis of single-atom catalysts as well as metal-free carbocatalysts for organic reactions

jbxi@wit.edu.cn

Received Date: 29 August 2022
Revised Date: 23 October 2022
Accepted Date: 26 October 2022
Available Online: 30 October 2022

Figures(10)

Metal-based catalysis, including homogeneous and heterogeneous catalysis, plays a significant role in the modern chemical industry. Heterogeneous catalysis is widely used due to the high efficiency, easy catalyst separation and recycling. However, the metal-utilization efficiency for conventional heterogeneous catalysts needs further improvement compared to homogeneous catalyst. To tackle this, the pursing of heterogenizing homogeneous catalysts has always been attractive but challenging. As a recently emerging class of catalytic material, single-atom catalysts (SACs) are expected to bridge homogeneous and heterogeneous catalytic process in organic reactions and have arguably become the most active new frontier in catalysis field. In this review, a brief introduction and development history of single-atom catalysis and SACs involved organic reactions are documented. In addition, recent advances in SACs and their practical applications in organic reactions such as oxidation, reduction, addition, coupling reaction, and other organic reactions are thoroughly reviewed. To understand structure-property relationships of single-atom catalysis in organic reactions, active sites or coordination structure, metal atom-utilization efficiency (e.g., turnover frequency, TOF calculated based on active metal) and catalytic performance (e.g., conversion and selectivity) of SACs are comprehensively summarized. Furthermore, the application limitations, development trends, future challenges and perspective of SAC for organic reaction are discussed.
- Single-atom catalysis,
- Active site,
- Metal utilization,
- Organic reaction,
- Catalytic performance
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