Citation: Lisha Chen, Qianqian Tang, Shihao Wu, Longshuai Zhang, Lifang Feng, Yuan Wang, Yiling Xie, Yan Li, Jian-Ping Zou, Sheng-Lian Luo. Covalent coupling promoting charge transport of CdSeTe/UiO-66 for boosting photocatalytic CO₂ reduction[J]. Chinese Chemical Letters, ;2023, 34(6): 107903. doi: 10.1016/j.cclet.2022.107903 shu

Covalent coupling promoting charge transport of CdSeTe/UiO-66 for boosting photocatalytic CO₂ reduction

Lisha Chen ^a ,
Qianqian Tang ^b ,
Shihao Wu ^b ,
Longshuai Zhang ^{b, *,} ,
Lifang Feng ^b ,
Yuan Wang ^c ,
Yiling Xie ^c ,
Yan Li ^c ,
Jian-Ping Zou ^{a, b, *,} ,
Sheng-Lian Luo ^{a, b}

a.
Key Laboratory of Poyang Lake Environment and Resource Utilization of Ministry of Education, School of Resources & Environment, Nanchang University, Nanchang 330031, China
b.
Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle, Nanchang Hangkong University, Nanchang 330063, China
c.
School of Chemistry & Molecular Engineering, East China University of Science and Technology, Shanghai 200237, China

Zhang1990@163.com

zjp_112@126.com

Received Date: 20 July 2022
Revised Date: 21 September 2022
Accepted Date: 10 October 2022
Available Online: 14 October 2022

Figures(5)

Quantum dots (QDs) based heterojunction is a candidate for the photocatalytic CO₂ reduction, owing to the large extinction coefficient and easy modification of band structures. However, the van der Waals interaction causes the large charge resistance and strong recombination centers between QDs and host materials, which makes the poor photocatalytic performance. Herein, a covalent bonded CdSeTe QDs and NH₂-UiO-66 heterojunction (NUC-x) is constructed through an acylamino (-CONH-). The results indicate that the acylamino between NH₂-UiO-66 and CdSeTe QDs can serve as the transfer channels for the photogenerated charges and stabilize the QDs. The optimized NUC-1200 achieved a CO generation rate of 228.68 µmol/g, which is 13 and 4 times higher than that of NH₂-UiO-66 and CdSeTe QDs, respectively. This work provides a new avenue for efficient and stable photocatalysis of QDs.
- Covalent coupling,
- CO₂ reduction,
- MOFs,
- Quantum dots,
- Photocatalytic
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沈阳化工大学材料科学与工程学院沈阳 110142

Covalent coupling promoting charge transport of CdSeTe/UiO-66 for boosting photocatalytic CO2 reduction

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通讯作者: 陈斌, bchen63@163.com

Covalent coupling promoting charge transport of CdSeTe/UiO-66 for boosting photocatalytic CO₂ reduction