Citation: Bao Li, Bobo Cao, Xinxin Zhou, Zhuangzhuang Zhang, Dongmei Dai, Mengmin Jia, Dai-Huo Liu. Pre-constructed SEI on graphite-based interface enables long cycle stability for dual ion sodium batteries[J]. Chinese Chemical Letters, ;2023, 34(7): 107832. doi: 10.1016/j.cclet.2022.107832 shu

Pre-constructed SEI on graphite-based interface enables long cycle stability for dual ion sodium batteries

Collaborative Innovation Center of Henan Province for Green Manufacturing of Fine Chemicals, Key Laboratory of Green Chemical Media and Reactions, Ministry of Education, School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang 453007, China

daidongmei@htu.edu.cn

jiamengmin@htu.edu.cn

liudaihuo@htu.edu.cn

Received Date: 21 June 2022
Revised Date: 8 August 2022
Accepted Date: 14 September 2022
Available Online: 17 September 2022

Figures(4)

Lithium batteries have been widely used in all over the world for its high energy density, long-term cycle stability. While the resources of lithium metal and transition metal are limited, which restrict their applications in the grid energy storage. Dual ion sodium batteries (DISBs) possess higher energy density, especially owning high power density for its higher operating voltage (> 4.5 V). Nevertheless, the poor oxidation tolerance of carbonate electrolyte and the co-intercalation of solvents accompanied with anions are main obstacles to make the DISBs commercialization. Herein, a physical barrier (artificial SEI film) is pre-constructed in the Na||graphite batteries to solve these thorny problems. With the CSMG (covered SEI on modified graphite), batteries deliver higher capacity 40 mAh/g even under the current density of 300 mA/g and the capacity retention maintains very well after 100 cycles at a high operating voltage. Moreover, the function mechanism was revealed by in-situ XRD, demonstrating that the pre-constructed SEI can effectively suppress the irreversible phase transition and exfoliation of graphite, resulting from the co-intercalation of anions. Additionally, the work voltage windows of carbonate electrolyte are significantly broadened by establishing electrode/electrolyte interphase. This method opens up an avenue for the practical application of DISBs on the grid energy storage and other fields.
- Dual ion sodium batteries,
- Carbonate electrolyte,
- High voltage,
- Anion co-intercalation,
- Pre-constructed SEI
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