Citation: Lejian Yu, Miao Wang, Xipeng Li, Xu Hou. Thermally responsive ionic transport system reinforced by aligned functional carbon nanotubes backbone[J]. Chinese Chemical Letters, ;2023, 34(7): 107785. doi: 10.1016/j.cclet.2022.107785 shu

Thermally responsive ionic transport system reinforced by aligned functional carbon nanotubes backbone

Lejian Yu ^a ,
Miao Wang ^b, ,
Xipeng Li ^a ,
Xu Hou ^{a, c, d, **,}

a.
State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, China
b.
The Higher Educational Key Laboratory for Biomedical Engineering of Fujian Province, Research Center of Biomedical Engineering of Xiamen, Department of Biomaterials, College of Materials, Xiamen University, Xiamen 361005, China
c.
Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials Research, Jiujiang Research Institute, College of Physical Science and Technology, Xiamen University, Xiamen 361005, China
d.
Innovation Laboratory for Sciences and Technologies of Energy Materials of Fujian Province (IKKEM), Xiamen 361005, China

^**

miaowang@xmu.edu.cn

houx@xmu.edu.cn

Received Date: 1 July 2022
Revised Date: 21 July 2022
Accepted Date: 24 August 2022
Available Online: 27 August 2022

Figures(4)

Ion transport plays an important role in energy conversion, biosensors, and a variety of biological processes. Carbon nanotubes, especially for the carbon nanotubes arrays with controlled vertically aligned structures, have displayed great potential as a promising material for regulating ion transport behaviors in the applications of the nanofluidic devices and osmotic energy conversion. Herein, we demonstrate the thermo-controlled ion transport system through the vertically aligned multiwall carbon nanotubes arrays membrane modified by the thermo-responsive hydrogel in a simple and reliable way. The functional carbon nanotubes backbone with the inherent surface charge and interstitial channels structure renders the system improved ion transport behaviors and well controlled switching property by thermo. Based on the integrated properties, the energy output from osmotic power in this system could be regulated by the reversible temperature switches. Moreover, it can realize a higher osmotic energy conversion property regulated by the thermos, which may extend the practical application in the future. The system that combines intelligent response with controlled ion transport behaviors and potential osmotic energy utilizations presents a valuable paradigm for the use of carbon nanotubes and hydrogel composite materials and provides a promising way for applications of nanofluidic devices.
- Carbon nanotubes arrays,
- Ion transport system,
- Interstitial channels,
- Thermo-controlled,
- Osmotic energy
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1.
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